PLANAR LASER-INDUCED-FLUORESCENCE IMAGING MEASUREMENTS OF OH AND HYDROCARBON FUEL FRAGMENTS IN HIGH-PRESSURE SPRAY-FLAME COMBUSTION

被引:43
作者
ALLEN, MG [1 ]
MCMANUS, KR [1 ]
SONNENFROH, DM [1 ]
PAUL, PH [1 ]
机构
[1] SANDIA NATL LABS,COMBUST RES FACIL,LIVERMORE,CA 94551
来源
APPLIED OPTICS | 1995年 / 34卷 / 27期
关键词
FLUORESCENCE; COMBUSTION DIAGNOSTICS; HIGH-PRESSURE COMBUSTION; OH; POLYCYCLIC AROMATIC HYDROCARBON; SPRAY FLAME;
D O I
10.1364/AO.34.006287
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Planar laser-induced fluorescence images of OH have been obtained in liquid-fueled spray flames burning heptane, ethanol, and methanol over a range of pressures from 0.1 to 1.0 MPa. In addition to the OH fluorescence, a nonresonant fluorescence interference that increased rapidly with pressure was detected. Examination of the spectrum of this interference indicates that it arises from hydrocarbon fuel-fragment species in the fuel-rich zones of the flame. The pressure dependence of the fluorescence signal is examined in both steady-state and time-dependent analyses, and a model for evaluation of pressure effects and quenching variations in quantitative imaging measurements in nonpremixed flame environments is presented. The results indicate that increased combustor pressure results in a rapid rise of the volume fraction of hydrocarbon fragments and a decrease in the OH volume fraction.
引用
收藏
页码:6287 / 6300
页数:14
相关论文
共 40 条
[11]  
BATTLES BE, 1991, 22ND AIAA FLUID DYN
[12]  
BATTLES BE, 1994, 32ND AER SCI M AM I
[13]  
BONIG M, 1990, 23 S INT COMB COMB I, P1581
[14]  
Calvert J. G., 1966, PHOTOCHEMISTRY
[15]   SATURATED FLUORESCENCE MEASUREMENTS OF THE HYDROXYL RADICAL IN LAMINAR HIGH-PRESSURE C2H6/O2/N2 FLAMES [J].
CARTER, CD ;
KING, GB ;
LAURENDEAU, NM .
APPLIED OPTICS, 1992, 31 (10) :1511-1522
[16]  
CIAJOLO A, 1982, 19TH S INT COMB, P1369
[17]   SIMULTANEOUS ONE-DIMENSIONAL VISUALIZATION OF OH, POLYCYCLIC AROMATIC-HYDROCARBONS, AND SOOT IN A LAMINAR DIFFUSION FLAME [J].
CIGNOLI, F ;
BENECCHI, S ;
ZIZAK, G .
OPTICS LETTERS, 1992, 17 (04) :229-231
[18]  
DRAKE MC, 1991, 23 S INT COMB P, P387
[19]  
FLOWER WL, 1986, 21ST S INT COMB PITT, P1115
[20]   PREDISSOCIATION LIFETIMES OF OH A2-SIGMA+ (V'=3) OBTAINED FROM OPTICAL OPTICAL DOUBLE-RESONANCE LINEWIDTH MEASUREMENTS [J].
GRAY, JA ;
FARROW, RL .
JOURNAL OF CHEMICAL PHYSICS, 1991, 95 (10) :7054-7060