INTERACTION OF 1-BUTENE AND NORMAL-BUTANE WITH A SULFATE-PROMOTED IRON-OXIDE

被引:21
作者
LEE, JS
YEOM, MH
PARK, DS
机构
[1] Department of Chemical Engineering, Pohang Institute of Science and Technology, Research Institute of Industrial Science and Technology, Pohang
关键词
D O I
10.1016/0021-9517(90)90004-4
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Interactions of sulfate-promoted iron oxide SO2-4Fe2O3 with 1-butene and n-butane were investigated by means of infrared spectroscopy and temperature-programmed desorption/reaction coupled with mass spectrometry. By reacting with the sulfate ion, 1-butene adsorbed on SO42-Fe2O3 promoted sulfate decomposition. In contrast, adsorbed n-butane desorbed readily upon heating above 320 K. Implications of these findings in catalysis by this material are discussed. © 1990.
引用
收藏
页码:361 / 369
页数:9
相关论文
共 20 条
[11]   A RELATION BETWEEN OXIDATION-STATE OF SULFUR AND ACIDIC PROPERTY OF IRON-OXIDE CONTAINING SULFUR [J].
NAGASE, Y ;
JIN, T ;
HATTORI, H ;
YAMAGUCHI, T ;
TANABE, K .
BULLETIN OF THE CHEMICAL SOCIETY OF JAPAN, 1985, 58 (03) :916-918
[12]   CONVERSION OF METHANE-ETHYLENE MIXTURES OVER SULFATE-TREATED ZIRCONIA CATALYSTS [J].
SCURRELL, MS .
APPLIED CATALYSIS, 1987, 34 (1-2) :109-117
[13]  
SHEPPARD N, 1962, Q REV CHEM SOC, V6, P1
[14]   ENHANCED CATALYTIC ACTIVITY OF SPECIALLY PREPARED FE2O3 FOR THE ISOMERIZATION OF BUT-1-ENE AND CYCLOPROPANE AND THE DEHYDRATION OF BUTAN-2-O1 [J].
TANABE, K ;
KAYO, A ;
YAMAGUCHI, T .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1981, (12) :602-603
[15]  
TANABE K, 1989, SUCCESSFUL DESIGN CA, P99
[16]  
YAMAGUCHI T, 1986, J PHYS CHEM-US, V90, P3148, DOI 10.1021/j100405a022
[17]  
YAMAMOTO M, 1985, J CHEM SOC JAPAN, V5, P838
[18]   DEACTIVATION OF H-MORDENITE AND ZRO2/SO42- DURING NORMAL-BUTANE ISOMERIZATION [J].
YORI, JC ;
LUY, JC ;
PARERA, JM .
APPLIED CATALYSIS, 1989, 46 (01) :103-112
[19]  
[No title captured]
[20]  
[No title captured]