NATURE OF COARSE NITRATE PARTICLES IN THE ATMOSPHERE - A SINGLE, PARTICLE APPROACH

被引:78
作者
WU, PM
OKADA, K
机构
[1] Meteorological Research Institute, Tsukuba, Ibaraki
关键词
DUST PARTICLES; SEA-SALT PARTICLES; HETEROGENEOUS REACTION; NITRATE FORMATION; INDIVIDUAL PARTICLE; ELECTRON MICROSCOPY;
D O I
10.1016/1352-2310(94)90473-1
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Aerosol particles were collected in Nagoya, a coastal city of Japan. Individual nitrate-containing particles were identified with a vapor-deposited thin film method by electron microscopy. Elemental composition of individual coarse nitrate-containing particles was determined with X-ray spectrometry. Nitrate was detected in the coarse particles in all the samples. It was observed that chemical modification of sea-salt particles by nitric acid occurred frequently in the coastal urban area. It is found that nitrate also existed on the surface of dust particles during the period of ''Kosa'' phenomenon, a yellow sand storm originating from East Asian deserts or loess areas observed in Japan. Nitrate formation through heterogeneous reactions on the dust particles may provide a removal mechanism for the nitrogen oxides in the atmosphere in ''Kosa'' phenomenon.
引用
收藏
页码:2053 / 2060
页数:8
相关论文
共 36 条
[21]  
Lundgren D A, 1970, J Air Pollut Control Assoc, V20, P603
[22]   NITRATE FORMATION ON SEA-SALT AND MINERAL PARTICLES - A SINGLE-PARTICLE APPROACH [J].
MAMANE, Y ;
GOTTLIEB, J .
ATMOSPHERIC ENVIRONMENT PART A-GENERAL TOPICS, 1992, 26 (09) :1763-1769
[23]   HETEROGENEOUS REACTIONS OF MINERALS WITH SULFUR AND NITROGEN-OXIDES [J].
MAMANE, Y ;
GOTTLIEB, J .
JOURNAL OF AEROSOL SCIENCE, 1989, 20 (03) :303-311
[24]   ON THE NATURE OF NITRATE PARTICLES IN A COASTAL URBAN AREA [J].
MAMANE, Y ;
MEHLER, M .
ATMOSPHERIC ENVIRONMENT, 1987, 21 (09) :1989-1994
[25]  
NISHIKAWA M, 1991, TENKI, V38, P225
[26]  
NISHIKAWA M, 1989, ANAL CARBONACEOUS MA, P58
[27]   X-RAY SPECTROMETRY OF INDIVIDUAL ASIAN DUST-STORM PARTICLES OVER THE JAPANESE ISLANDS AND THE NORTH PACIFIC-OCEAN [J].
OKADA, K ;
NARUSE, H ;
TANAKA, T ;
NEMOTO, O ;
IWASAKA, Y ;
WU, PM ;
ONO, A ;
DUCE, RA ;
UEMATSU, M ;
MERRILL, JT ;
ARAO, K .
ATMOSPHERIC ENVIRONMENT PART A-GENERAL TOPICS, 1990, 24 (06) :1369-1378
[29]   FEATURES OF INDIVIDUAL ASIAN DUST-STORM PARTICLES COLLECTED AT NAGOYA, JAPAN [J].
OKADA, K ;
KOBAYASHI, A ;
IWASAKA, Y ;
NARUSE, H ;
TANAKA, T ;
NEMOTO, O .
JOURNAL OF THE METEOROLOGICAL SOCIETY OF JAPAN, 1987, 65 (03) :515-521
[30]  
TAMAKA S, 1986, J CHEM SOC JAPAN, V5, P713