NONLINEAR-OPTICAL RESPONSE OF C-60 MOLECULES

被引：15

作者：

HARIGAYA, K

ABE, S

机构：

[1] ELECTROTECH LAB,1-1-4 UMEZONO,TSUKUBA 305,JAPAN

[2] UNIV SHEFFIELD,DEPT PHYS,SHEFFIELD S3 7RH,S YORKSHIRE,ENGLAND

来源：

JOURNAL OF LUMINESCENCE | 1994年 / 60-1卷

关键词：

D O I：

10.1016/0022-2313(94)90170-8

中图分类号：

O43 [光学];

学科分类号：

070207 ; 0803 ;

摘要：

The third-order nonlinear optical susceptibility chi(3) of the fullerene C60 is studied theoretically. A free-electron model yields chi(3) magnitudes which are in agreement with experiment. Coulomb interactions reduce chi(3) by an order of magnitude, while local-field corrections can be invoked to recover the agreement.

引用

收藏

页码：380 / 382

页数：3

相关论文

共 9 条

[1] COLLECTIVE PLASMON EXCITATIONS IN C60 CLUSTERS [J].

BERTSCH, GF ;

BULGAC, A ;

TOMANEK, D ;

WANG, Y .

PHYSICAL REVIEW LETTERS, 1991, 67 (19) :2690-2693

[2] DISPERSION OF THE 3RD-ORDER NONLINEAR OPTICAL SUSCEPTIBILITY IN C-60 CALCULATED WITH A TIGHT-BINDING MODEL [J].

HARIGAYA, K ;

ABE, S .

JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS, 1992, 31 (7A) :L887-L889

[3] OFF-RESONANT NONLINEAR OPTICAL-PROPERTIES OF C60 STUDIED BY DEGENERATE 4-WAVE-MIXING [J].

KAFAFI, ZH ;

LINDLE, JR ;

PONG, RGS ;

BARTOLI, FJ ;

LINGG, LJ ;

MILLIKEN, J .

CHEMICAL PHYSICS LETTERS, 1992, 188 (5-6) :492-496

[4] DISPERSION OF THE 3RD-ORDER OPTICAL NONLINEARITY OF C-60 - A 3RD-HARMONIC GENERATION STUDY [J].

METH, JS ;

VANHERZEELE, H ;

WANG, Y .

CHEMICAL PHYSICS LETTERS, 1992, 197 (1-2) :26-31

[5] DENSITY-FUNCTIONAL-BASED LINEAR AND NONLINEAR POLARIZABILITIES OF FULLERENE AND BENZENE MOLECULES [J].

QUONG, AA ;

PEDERSON, MR .

PHYSICAL REVIEW B, 1992, 46 (19) :12906-12909

[6] ELECTRONIC-STRUCTURE AND NONLINEAR OPTICAL-PROPERTIES OF THE FULLERENES C-60 AND C-70 - A VALENCE-EFFECTIVE-HAMILTONIAN STUDY [J].

SHUAI, ZG ;

BREDAS, JL .

PHYSICAL REVIEW B, 1992, 46 (24) :16135-16141

[7]

TAKAHASHI A, PREPRINT

[8] HYPERPOLARIZABILITY OF THE C60 FULLERENE CLUSTER [J].

WANG, Y ;

BERTSCH, GF ;

TOMANEK, D .

ZEITSCHRIFT FUR PHYSIK D-ATOMS MOLECULES AND CLUSTERS, 1993, 25 (02) :181-184

[9]

WESTIN E, 1992, INT J MOD PHYS B, V23, P3893