Two-dimensional J-resolved and SUPERCOSY NMR experiments in the solid state

被引:10
作者
Kolodziejski, Waclaw [1 ]
Klinowski, Jacek [1 ]
机构
[1] Univ Cambridge, Dept Chem, Cambridge CB2 1EW, England
关键词
solid-state NMR; two-dimensional NMR; J-resolved; COSY; Q(8)M(8);
D O I
10.1016/0926-2040(92)90008-W
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Two 2D experiments, novel to solid-state NMR, are demonstrated using the trimethylsilyl ester of cubic octameric silicate (Q(8)M(8)). J-Resolved C-13 NMR with BLEW-12 proton homonuclear decoupling reveals the scalar C-13-H-1 couplings and Si-29 SUPERCOSY the connectivities of silicon atoms in the distorted Q(8) cube.
引用
收藏
页码:41 / 44
页数:4
相关论文
共 26 条
[1]   THE OBSERVATION OF TWO-DIMENSIONAL NMR-SPECTRA OF CRYSTALLINE SOLIDS - THE P-31 CP-MAS COSY AND J-RESOLVED SPECTRA OF A PHOSPHINE COMPLEX OF HG(II) [J].
ALLMAN, T .
JOURNAL OF MAGNETIC RESONANCE, 1989, 83 (03) :637-642
[2]   MONITORING ORGANIC-PRODUCTS OF CATALYTIC REACTIONS ON ZEOLITES BY 2-DIMENSIONAL J-RESOLVED SOLID-STATE NMR [J].
ANDERSON, MW ;
KLINOWSKI, J .
CHEMICAL PHYSICS LETTERS, 1990, 172 (3-4) :275-278
[3]   THE DETECTION OF CONNECTIVITIES OF RARE SPIN-1/2 NUCLEI IN THE SOLID-STATE USING NATURAL ABUNDANCE SAMPLES - C-13 AND SI-29 INADEQUATE AND COSY TYPE EXPERIMENTS [J].
BENN, R ;
GRONDEY, H ;
BREVARD, C ;
PAGELOT, A .
JOURNAL OF THE CHEMICAL SOCIETY-CHEMICAL COMMUNICATIONS, 1988, (02) :102-103
[4]   A MULTIPHASE ONE-DIMENSIONAL AND TWO-DIMENSIONAL P-31 NMR INVESTIGATION OF P4S7 [J].
BJORHOLM, T .
CHEMICAL PHYSICS LETTERS, 1988, 143 (03) :259-262
[5]   LOW-POWER MULTIPULSE LINE NARROWING IN SOLID-STATE NMR [J].
BURUM, DP ;
LINDER, M ;
ERNST, RR .
JOURNAL OF MAGNETIC RESONANCE, 1981, 44 (01) :173-188
[6]  
ENGELHARDT G, 1982, Z CHEM, V22, P314
[7]  
Engelhardt G., 1987, HIGH RESOLUTION SOLI
[8]   DETERMINATION OF 3-DIMENSIONAL LATTICE CONNECTIVITIES IN ZEOLITES USING NATURAL-ABUNDANCE SI-29 TWO-DIMENSIONAL NMR AND THE DIRECT OBSERVATION OF SI-29-O-SI-29 COUPLINGS [J].
FYFE, CA ;
GIES, H ;
FENG, Y ;
KOKOTAILO, GT .
NATURE, 1989, 341 (6239) :223-225
[9]   NATURAL-ABUNDANCE 2-DIMENSIONAL SI-29 MAS NMR INVESTIGATION OF THE 3-DIMENSIONAL BONDING CONNECTIVITIES IN THE ZEOLITE CATALYST ZSM-5 [J].
FYFE, CA ;
GRONDEY, H ;
FENG, Y ;
KOKOTAILO, GT .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1990, 112 (24) :8812-8820
[10]   NATURAL-ABUNDANCE 2-DIMENSIONAL SOLID-STATE SI-29 NMR INVESTIGATIONS OF 3-DIMENSIONAL LATTICE CONNECTIVITIES IN ZEOLITE STRUCTURES [J].
FYFE, CA ;
FENG, Y ;
GIES, H ;
GRONDEY, H ;
KOKOTAILO, GT .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1990, 112 (09) :3264-3270