MEASUREMENT OF THE LARGE OPTICAL NONLINEARITY OF NICKEL DITHIOLENE DOPED POLYMERS

被引:12
作者
WINTER, CS
MANNING, RJ
OLIVER, SN
HILL, CAS
机构
[1] BT Laboratories, Ipswich, IP5 7RE, Martlesham Heath
关键词
D O I
10.1016/0030-4018(92)90345-R
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The nonlinear refractive indices and the two-photon absorption coefficients of films of three nickel dithiolene complexes dissolved at various concentrations in a polymethylmethacrylate (PMMA) host were measured using the Z-scan technique. Nonlinear refractive indices up to 10(-8) cm2/kW were observed. The device-based figure of merit. DELTA-n(sat)/alpha-lambda, was found to be greater than 2. At high doping concentrations two-photon absorption increased more rapidly with concentration than the nonlinear refractive index. reducing the ratio of the Re-chi(3) to Im-chi(3) below that acceptable for devices, thus limiting the maximum usable concentration of the guest in a PMMA host.
引用
收藏
页码:139 / 143
页数:5
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