STRETCHED-EXPONENTIAL RELAXATION AT A SELF-SIMILAR SURFACE

被引:28
作者
HALSEY, TC [1 ]
LEIBIG, M [1 ]
机构
[1] UNIV CHICAGO, DEPT PHYS, CHICAGO, IL 60637 USA
来源
PHYSICAL REVIEW A | 1991年 / 43卷 / 12期
关键词
D O I
10.1103/PhysRevA.43.7087
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
The double-layer impedance at a rough electrode can be related to properties of random walks near the surface of that electrode. We apply this method to the calculation of the double-layer impedance at a self-similar electrode in two dimensions. We find that the impedance at a self-similar surface shows stretched-exponential behavior. At high frequencies, this behavior is similar to the experimentally observed constant phase-angle behavior, with an exponent determined by the multifractal properties of the surface.
引用
收藏
页码:7087 / 7090
页数:4
相关论文
共 34 条
[21]   SELF-AFFINE FRACTAL MODEL FOR A METAL-ELECTROLYTE INTERFACE [J].
KAPLAN, T ;
GRAY, LJ ;
LIU, SH .
PHYSICAL REVIEW B, 1987, 35 (10) :5379-5381
[22]   IMPEDANCE OF FRACTAL INTERFACES - NEW DATA ON THE VONKOCH MODEL [J].
KEDDAM, M ;
TAKENOUTI, H .
ELECTROCHIMICA ACTA, 1988, 33 (03) :445-448
[23]  
LEMEHAUTE A, 1983, SOLID STATE IONICS, V9-10, P17, DOI 10.1016/0167-2738(83)90207-2
[24]   FRACTAL MODEL FOR THE AC RESPONSE OF A ROUGH INTERFACE [J].
LIU, SH .
PHYSICAL REVIEW LETTERS, 1985, 55 (05) :529-532
[25]   DIFFUSION-CONTROLLED CLUSTER FORMATION IN 2-6-DIMENSIONAL SPACE [J].
MEAKIN, P .
PHYSICAL REVIEW A, 1983, 27 (03) :1495-1507
[26]   RANDOM-WALK SIMULATION OF THE RESPONSE OF IRREGULAR OR FRACTAL INTERFACES AND MEMBRANES [J].
MEAKIN, P ;
SAPOVAL, B .
PHYSICAL REVIEW A, 1991, 43 (06) :2993-3004
[27]   FRACTAL DIMENSION AND FRACTIONAL POWER FREQUENCY-DEPENDENT IMPEDANCE OF BLOCKING ELECTRODES [J].
NYIKOS, L ;
PAJKOSSY, T .
ELECTROCHIMICA ACTA, 1985, 30 (11) :1533-1540
[28]   MODELS OF HIERARCHICALLY CONSTRAINED DYNAMICS FOR GLASSY RELAXATION [J].
PALMER, RG ;
STEIN, DL ;
ABRAHAMS, E ;
ANDERSON, PW .
PHYSICAL REVIEW LETTERS, 1984, 53 (10) :958-961
[29]   STOCHASTIC-MODEL FOR DIELECTRIC-BREAKDOWN [J].
PIETRONERO, L ;
WIESMANN, HJ .
JOURNAL OF STATISTICAL PHYSICS, 1984, 36 (5-6) :909-916