NONLINEAR OPTICAL-RESPONSE OF C-60 AND C-70

被引:77
作者
NEHER, D
STEGEMAN, GI
TINKER, FA
PEYGHAMBARIAN, N
机构
[1] UNIV CENT FLORIDA,CTR RES ELECTROOPT & LASERS,ORLANDO,FL 32826
[2] UNIV ARIZONA,DEPT PHYS,TUCSON,AZ 85721
[3] UNIV ARIZONA,CTR OPT SCI,TUCSON,AZ 85721
关键词
D O I
10.1364/OL.17.001491
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
Second-order hyperpolarizibilities gamma of the buckminsterfullerenes C70 at three different wavelengths were determined by third-harmonic generation in a toluene solution and compared with those of C60. Strong effects with gamma exceeding 5 x 10(-32) esu were observed in the three-photon resonant regime. The nonresonant measurements indicate a negative real hyperpolarizibility in C70 and a positive gamma for C60, both of the order of 10(-33) esu.
引用
收藏
页码:1491 / 1493
页数:3
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