PREPARATION OF (BA, SR)TIO3 THIN-FILMS BY CHEMICAL-VAPOR-DEPOSITION USING LIQUID SOURCES

被引:43
作者
KAWAHARA, T [1 ]
YAMAMUKA, M [1 ]
MAKITA, T [1 ]
TSUTAHARA, K [1 ]
YUUKI, A [1 ]
ONO, K [1 ]
MATSUI, Y [1 ]
机构
[1] MITSUBISHI ELECTR CORP,KITA ITAMI WORKS,ITAMI,HYOGO 664,JAPAN
来源
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS SHORT NOTES & REVIEW PAPERS | 1994年 / 33卷 / 10期
关键词
LSI; CVD; CAPACITOR; BST; DPM; DIELECTRIC CONSTANT; LEAKAGE CURRENT; DIELECTRIC LOSS; STEP COVERAGE;
D O I
10.1143/JJAP.33.5897
中图分类号
O59 [应用物理学];
学科分类号
摘要
Thin films of (Ba, Sr)TiO3 with high dielectric constant were prepared on Pt/SiO2/Si substrates of 6-inch-diameter by chemical vapor deposition using liquid sources. Ba(DPM)(2) and Sr(DPM)(2) dissolved into tetrahydrofuran were vaporized in a vaporizer at 523 K, and Ti(O-i-C3H7)(4) was bubbled at 313 K. The mixture of the source vapors with O-2 and N2O was supplied to the reactor (10 Torr) at uniform velocities through a shower-type nozzle, which realized uniform profiles in the deposited film thickness and composition. The electrical properties are significantly influenced by the film composition, and the typical properties obtained for a 800-Angstrom-thick film prepared at the substrate temperature of 823 K are an equivalent SiO2 thickness t(eq) of 5.2 Angstrom, a leakage current J(L) of 2.4 x 10(-6) A/cm(2) (at 1.65 V), and a dielectric loss tan delta of 0.07.
引用
收藏
页码:5897 / 5902
页数:6
相关论文
共 12 条
[1]   SURFACE-REACTION RATE DURING ZRO2 THIN-FILM FORMATION BY MOCVD - STEP COVERAGE ON MICRO-TRENCHES [J].
AKIYAMA, Y ;
IMAISHI, N .
KAGAKU KOGAKU RONBUNSHU, 1992, 18 (02) :212-218
[2]   SPECTROSCOPIC STUDY ON A DISCHARGE PLASMA OF MOCVD SOURCE GASES FOR HIGH-TC SUPERCONDUCTING FILMS [J].
HARIMA, H ;
OHNISHI, H ;
HANAOKA, K ;
TACHIBANA, K ;
KOBAYASHI, M ;
HOSHINOUCHI, S .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS BRIEF COMMUNICATIONS & REVIEW PAPERS, 1990, 29 (10) :1932-1938
[3]   DIELECTRIC-PROPERTIES OF (BA, SR)TIO3 THIN-FILMS DEPOSITED BY RF-SPUTTERING [J].
HORIKAWA, T ;
MIKAMI, N ;
MAKITA, T ;
TANIMURA, J ;
KATAOKA, M ;
SATO, K ;
NUNOSHITA, M .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS SHORT NOTES & REVIEW PAPERS, 1993, 32 (9B) :4126-4130
[4]   REACTION-MECHANISM OF CHEMICAL VAPOR-DEPOSITION USING TETRAETHYLORTHOSILICATE AND OZONE AT ATMOSPHERIC-PRESSURE [J].
KAWAHARA, T ;
YUUKI, A ;
MATSUI, Y .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS SHORT NOTES & REVIEW PAPERS, 1992, 31 (9A) :2925-2930
[5]   A STUDY ON THE BEHAVIOR OF SIO2 FILM PRECURSORS WITH TRENCH DEPOSITION METHOD FOR SIH4/O2 LOW-PRESSURE CHEMICAL VAPOR-DEPOSITION [J].
KAWAHARA, T ;
YUUKI, A ;
MATSUI, Y .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS BRIEF COMMUNICATIONS & REVIEW PAPERS, 1991, 30 (03) :431-436
[6]   Y-BA-CU-O SUPERCONDUCTING FILMS WITH HIGH-JC VALUES BY MOCVD USING BA-ADDITION PRODUCTS [J].
MATSUNO, S ;
UCHIKAWA, F ;
YOSHIZAKI, K .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS, 1990, 29 (06) :L947-L948
[7]  
MITSUI T, 1981, LANDOLTBORNSTEIN, V16, P59
[8]  
MIYASAKA Y, 1991, 7TH P INT S APPL FER, P121
[9]  
VANBUSKIRK PC, 1992, 8TH P INT S APPL FER, P340
[10]   STRUCTURAL AND ELECTRICAL CHARACTERIZATION OF SRTIO3 THIN-FILMS PREPARED BY METAL-ORGANIC CHEMICAL-VAPOR-DEPOSITION [J].
YAMAGUCHI, H ;
LESAICHERRE, PY ;
SAKUMA, T ;
MIYASAKA, Y ;
ISHITANI, A ;
YOSHIDA, M .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS SHORT NOTES & REVIEW PAPERS, 1993, 32 (9B) :4069-4073