CLOSE SIMILARITY OF THE ELECTRONIC-STRUCTURE AND ELECTRON CORRELATION IN GAS-PHASE AND SOLID C-60

被引:47
作者
KRUMMACHER, S
BIERMANN, M
NEEB, M
LIEBSCH, A
EBERHARDT, W
机构
[1] Institut fur Festkorperforschung der Forschungszentrum Julich GmbH, D-52425 Julich
来源
PHYSICAL REVIEW B | 1993年 / 48卷 / 11期
关键词
D O I
10.1103/PhysRevB.48.8424
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
We present a study of the electronic structure and electron correlation effects in gas-phase and solid C60 clusters. Direct in situ comparison of C 1s absorption spectra taken in the gas phase with those from solid C60 reveals a close similarity. This is also true for the shake-up satellites in the C 1s x-ray-photoelectron spectrum. The main conclusions are that solid-state interactions play only a minor role in this new material, and electron correlation effects are predominantly intramolecular.
引用
收藏
页码:8424 / 8429
页数:6
相关论文
共 20 条
[1]   THE SOFT-X-RAY SPECTROSCOPY UNDULATOR BEAMLINE AT NSLS-X1 [J].
EBERHARDT, W ;
RANDALL, KJ ;
FELDHAUS, J ;
BRADSHAW, AM ;
GARRETT, RF ;
KNOTEK, ML .
PHYSICA SCRIPTA, 1990, 41 (06) :745-748
[2]   HIGH-RESOLUTION ELECTRON-ENERGY-LOSS SPECTROSCOPY OF THIN-FILMS OF C60 ON SI(100) [J].
GENSTERBLUM, G ;
PIREAUX, JJ ;
THIRY, PA ;
CAUDANO, R ;
VIGNERON, JP ;
LAMBIN, P ;
LUCAS, AA ;
KRATSCHMER, W .
PHYSICAL REVIEW LETTERS, 1991, 67 (16) :2171-2174
[3]   FULLERENE TRIPLET-STATE PRODUCTION AND DECAY - R2PI PROBES OF C60 AND C70 IN A SUPERSONIC BEAM [J].
HAUFLER, RE ;
WANG, LS ;
CHIBANTE, LPF ;
JIN, CM ;
CONCEICAO, J ;
CHAI, Y ;
SMALLEY, RE .
CHEMICAL PHYSICS LETTERS, 1991, 179 (5-6) :449-454
[4]   GIANT PLASMON EXCITATION IN FREE C-60 AND C-70 MOLECULES STUDIED BY PHOTOIONIZATION [J].
HERTEL, IV ;
STEGER, H ;
DEVRIES, J ;
WEISSER, B ;
MENZEL, C ;
KAMKE, B ;
KAMKE, W .
PHYSICAL REVIEW LETTERS, 1992, 68 (06) :784-787
[5]  
HITCHCOCK A, 1981, J ELECTRON SPECTROSC, V18, P1
[6]   K-SHELL EXCITATION-SPECTRA OF CO, N2 AND O2 [J].
HITCHCOCK, AP ;
BRION, CE .
JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 1980, 18 (1-2) :1-21
[7]   SOLID C-60 - A NEW FORM OF CARBON [J].
KRATSCHMER, W ;
LAMB, LD ;
FOSTIROPOULOS, K ;
HUFFMAN, DR .
NATURE, 1990, 347 (6291) :354-358
[8]   POLARIZATION-WAVES AND VANDERWAALS COHESION OF C-60 FULLERITE [J].
LAMBIN, P ;
LUCAS, AA ;
VIGNERON, JP .
PHYSICAL REVIEW B, 1992, 46 (03) :1794-1803
[9]   VALENCE AND CORE PHOTOELECTRON-SPECTROSCOPY OF C60, BUCKMINSTERFULLERENE [J].
LICHTENBERGER, DL ;
NEBESNY, KW ;
RAY, CD ;
HUFFMAN, DR ;
LAMB, LD .
CHEMICAL PHYSICS LETTERS, 1991, 176 (02) :203-208
[10]  
LICHTENBERGER DL, 1991, MATER RES SOC SYMP P, V206, P673, DOI 10.1557/PROC-206-673