锂电池百篇论文点评(2020.02.01—2020.03.31)

被引：1

作者：

金周

张华

田孟羽

季洪祥

田丰

起文斌

武怿达

詹元杰

闫勇

俞海龙

贲留斌

刘燕燕

黄学杰

机构：

[1] 中国科学院物理研究所

来源：

储能科学与技术 | 2020年 / 9卷 / 03期

关键词：

锂电池; 正极材料; 负极材料; 电解质; 电池技术;

D O I：

10.19799/j.cnki.2095-4239.2020.0151

中图分类号：

TM912 [蓄电池];

学科分类号：

0808 ;

摘要：

本文是一篇近两个月的锂电池文献评述,以"lithium"和"batter*"为关键词检索了Web of Science从2020年2月1日至2020年3月31日上线的锂电池研究论文,共有3295篇,选择其中100篇加以评论。正极材料主要研究了层状氧化物,主要是高镍三元的衰减机理和如何通过表界面修饰加以改善,富锂和高电压钴酸锂也有一部分。负极材料研究侧重于金属锂负极和硅负极,其中金属锂负极可通过制备界面膜,电解液添加剂或改进集流体促进锂离子均匀沉积,减少枝晶形成;硅基负极则聚焦于制备复合材料来抑制体积膨胀和提高电子电导,进而提升库仑效率和循环稳定性。固态电解质研究主要涵盖了高电导硫化物和有机聚合物电解质,液态电解质则重点研究功能添加剂对界面层的作用。固态、锂硫、锂空等电池技术还处在早期阶段,研究人员致力于寻找合适的电极设计和制备方法,保持电极的电子、离子传输性能及反应可逆性。在测量和表征技术上,多种原位技术可以获取电极内部的形貌、锂元素分布,电位分布等信息在充放电过程中的动态变化,从而为机理研究和性能提升提供依据。理论模拟工作侧重于界面SEI形成机理分析,此外还有一些介观和宏观尺度的理论模型被提出,来理解实际使用中的动力学问题。

引用

页码：762 / 775

页数：14

共 20 条

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