Localized and delocalized excitons:: Resonant inelastic X-ray scattering in La2-xSrxNiO4 and La2-xSrxCuO4

被引:50
作者
Collart, E
Shukla, A
Rueff, JP
Leininger, P
Ishii, H
Jarrige, I
Cai, YQ
Cheong, SW
Dhalenne, G
机构
[1] Univ Paris 06, Inst Mineral & Phys Milieux Condenses, F-75252 Paris 05, France
[2] Chim Phys Lab, F-75231 Paris 05, France
[3] Natl Synchrotron Radiat Res Ctr, Hsinchu 30076, Taiwan
[4] Rutgers State Univ, Rutgers Ctr Emergent Mat, Piscataway, NJ 08854 USA
[5] Rutgers State Univ, Dept Phys & Astron, Piscataway, NJ 08854 USA
[6] Univ Paris 11, Lab PhysicoChim Etat Solide, F-91405 Orsay, France
关键词
D O I
10.1103/PhysRevLett.96.157004
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
The dynamics of doped charge in an antiferromagnetic lattice is central to the description of the insulator-metal transition that occurs on doping the parent high T-c compounds. In this work we use high resolution resonant inelastic x-ray scattering to investigate the dynamics of the charge-transfer exciton by measuring its energy dispersion in two prototype compounds, La2CuO4 and La2NiO4. We show that this behavior is radically different in the cuprate with respect to a system known to exhibit strong polaronic behavior, namely, the nickelate: the exciton is mobile in the cuprate while it is well localized in the nickelate. Using a simple Wannier-Mott model we can estimate the total hole plus electron effective mass in the cuprate to be 3.5 +/- 0.3m(e) which would exclude strong localization in the undoped cuprate.
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页数:4
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共 19 条
[11]   Polaronic behavior of undoped high-Tc cuprate superconductors from angle-resolved photoemission spectra -: art. no. 227002 [J].
Rösch, O ;
Gunnarsson, O ;
Zhou, XJ ;
Yoshida, T ;
Sasagawa, T ;
Fujimori, A ;
Hussain, Z ;
Shen, ZX ;
Uchida, S .
PHYSICAL REVIEW LETTERS, 2005, 95 (22)
[12]   Missing quasiparticles and the chemical potential puzzle in the doping evolution of the cuprate superconductors [J].
Shen, KM ;
Ronning, F ;
Lu, DH ;
Lee, WS ;
Ingle, NJC ;
Meevasana, W ;
Baumberger, F ;
Damascelli, A ;
Armitage, NP ;
Miller, LL ;
Kohsaka, Y ;
Azuma, M ;
Takano, M ;
Takagi, H ;
Shen, ZX .
PHYSICAL REVIEW LETTERS, 2004, 93 (26)
[13]   Polarized resonant inelastic x-ray scattering as an ultrafine probe of excited states of La2CuO4 [J].
Shukla, A ;
Calandra, M ;
Taguchi, M ;
Kotani, A ;
Vankó, G ;
Cheong, SW .
PHYSICAL REVIEW LETTERS, 2006, 96 (07)
[14]   Evidence for suppressed screening on the surface of high temperature La2-xSrxCuO4 and Nd2-xCexCuO4 superconductors -: art. no. 177002 [J].
Taguchi, M ;
Chainani, A ;
Horiba, K ;
Takata, Y ;
Yabashi, M ;
Tamasaku, K ;
Nishino, Y ;
Miwa, D ;
Ishikawa, T ;
Takeuchi, T ;
Yamamoto, K ;
Matsunami, M ;
Shin, S ;
Yokoya, T ;
Ikenaga, E ;
Kobayashi, K ;
Mochiku, T ;
Hirata, K ;
Hori, J ;
Ishii, K ;
Nakamura, F ;
Suzuki, T .
PHYSICAL REVIEW LETTERS, 2005, 95 (17)
[15]   ANISOTROPY OF THE CORE-HOLE RELAXATION IN X-RAY-ABSORPTION SPECTROSCOPY AS PROBED IN SQUARE-PLANAR CUPRATES [J].
TOLENTINO, H ;
MEDARDE, M ;
FONTAINE, A ;
BAUDELET, F ;
DARTYGE, E ;
GUAY, D ;
TOURILLON, G .
PHYSICAL REVIEW B, 1992, 45 (14) :8091-8096
[16]   Mott gap excitations and resonant inelastic x-ray scattering in doped cuprates [J].
Tsutsui, K ;
Tohyama, T ;
Maekawa, S .
PHYSICAL REVIEW LETTERS, 2003, 91 (11) :117001-117001
[17]   OPTICAL-SPECTRA OF LA2-XSRXCUO4 - EFFECT OF CARRIER DOPING ON THE ELECTRONIC-STRUCTURE OF THE CUO2 PLANE [J].
UCHIDA, S ;
IDO, T ;
TAKAGI, H ;
ARIMA, T ;
TOKURA, Y ;
TAJIMA, S .
PHYSICAL REVIEW B, 1991, 43 (10) :7942-7954
[18]   FREEZING ELECTRONIC CORRELATIONS BY POLARONIC INSTABILITIES IN DOPED LA2NIO4 [J].
ZAANEN, J ;
LITTLEWOOD, PB .
PHYSICAL REVIEW B, 1994, 50 (10) :7222-7225
[19]   Theory of excitons in the insulating Cu-O2 plane [J].
Zhang, FC ;
Ng, KK .
PHYSICAL REVIEW B, 1998, 58 (20) :13520-13525