Synthesis of nitrogen-doped hollow carbon nanospheres for CO2 capture

被引:224
作者
Feng, Shanshan [1 ,2 ]
Li, Wei [1 ,2 ]
Shi, Quan [1 ,2 ]
Li, Yuhui [1 ,2 ]
Chen, Junchen [1 ,2 ]
Ling, Yun [1 ,2 ]
Asiri, Abdullah M. [3 ,4 ]
Zhao, Dongyuan [1 ,2 ]
机构
[1] Fudan Univ, Dept Chem, Shanghai 200433, Peoples R China
[2] Fudan Univ, Adv Mat Lab, Shanghai 200433, Peoples R China
[3] King Abdulaziz Univ, Dept Chem, Jeddah 21589, Saudi Arabia
[4] King Abdulaziz Univ, Ctr Excellence Adv Mat Res, Jeddah 21589, Saudi Arabia
关键词
OXYGEN REDUCTION; ACTIVATED CARBON; ELECTROCHEMICAL PERFORMANCE; FUNCTIONAL-GROUPS; SPHERES; ADSORPTION; SUPERCAPACITORS; NANOSTRUCTURES; MICROSPHERES; FABRICATION;
D O I
10.1039/c3cc46492j
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Here, we report the synthesis of nitrogen-doped hollow carbon nanospheres (N-HCSs) via a two-step Stober method. The resultant N-HCSs possess a uniform size of similar to 220 nm, a high nitrogen loading content of 14.8 wt% and a high surface area of 767m(2) g(-1), as well as exhibit a considerable performance for CO2 capture with a capacity of 2.67 mmol g(-1) and a high selectivity in a mixture gas (N-2 or O-2).
引用
收藏
页码:329 / 331
页数:3
相关论文
共 33 条
[21]   Efficient electrocatalytic oxygen reduction over metal free-nitrogen doped carbon nanocapsules [J].
Shanmugam, Sangaraju ;
Osaka, Tetsuya .
CHEMICAL COMMUNICATIONS, 2011, 47 (15) :4463-4465
[22]   Hollow carbon spheres with a controllable shell structure [J].
Su, Fabing ;
Zhao, X. S. ;
Wang, Yong ;
Wang, Likui ;
Lee, Jim Yang .
JOURNAL OF MATERIALS CHEMISTRY, 2006, 16 (45) :4413-4419
[23]   Polyethylenimine loaded nanoporous carbon with ultra-large pore volume for CO2 capture [J].
Tang, Zhihong ;
Han, Zhuo ;
Yang, Guangzhi ;
Yang, Junhe .
APPLIED SURFACE SCIENCE, 2013, 277 :47-52
[24]   Study of CO2 adsorption in functionalized carbon [J].
Vargas, Diana P. ;
Giraldo, L. ;
Moreno-Pirajan, J. C. .
ADSORPTION-JOURNAL OF THE INTERNATIONAL ADSORPTION SOCIETY, 2013, 19 (2-4) :323-329
[25]   Self-Supported Construction of Uniform Fe3O4 Hollow Microspheres from Nanoplate Building Blocks [J].
Wang, Bao ;
Wu, Hao Bin ;
Zhang, Lei ;
Lou, Xiong Wen .
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2013, 52 (15) :4165-4168
[26]   Highly porous nitrogen-doped polyimine-based carbons with adjustable microstructures for CO2 capture [J].
Wang, Jiacheng ;
Senkovska, Irena ;
Oschatz, Martin ;
Lohe, Martin R. ;
Borchardt, Lars ;
Heerwig, Andreas ;
Liu, Qian ;
Kaskel, Stefan .
JOURNAL OF MATERIALS CHEMISTRY A, 2013, 1 (36) :10951-10961
[27]   Ion-exchanged route synthesis of Fe2N-N-doped graphitic nanocarbons composite as advanced oxygen reduction electrocatalyst [J].
Wang, Lei ;
Yin, Jie ;
Zhao, Lu ;
Tian, Chungui ;
Yu, Peng ;
Wang, Jianqiang ;
Fu, Honggang .
CHEMICAL COMMUNICATIONS, 2013, 49 (29) :3022-3024
[28]   Increasing Selective CO2 Adsorption on Amine-Grafted SBA-15 by Increasing Silanol Density [J].
Wang, Lifeng ;
Yang, Ralph T. .
JOURNAL OF PHYSICAL CHEMISTRY C, 2011, 115 (43) :21264-21272
[29]   A Controllable Synthesis of Rich Nitrogen-Doped Ordered Mesoporous Carbon for CO2 Capture and Supercapacitors [J].
Wei, Jing ;
Zhou, Dandan ;
Sun, Zhenkun ;
Deng, Yonghui ;
Xia, Yongyao ;
Zhao, Dongyuan .
ADVANCED FUNCTIONAL MATERIALS, 2013, 23 (18) :2322-2328
[30]   Functional Hollow Carbon Nanospheres by Latex Templating [J].
White, Robin J. ;
Tauer, Klaus ;
Antonietti, Markus ;
Titirici, Maria-Magdalena .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2010, 132 (49) :17360-17363