Non-plasmonic nanoantennas for surface enhanced spectroscopies with ultra-low heat conversion

被引:422
作者
Caldarola, Martin [1 ,2 ]
Albella, Pablo [3 ]
Cortes, Emiliano [3 ]
Rahmani, Mohsen [3 ]
Roschuk, Tyler [3 ]
Grinblat, Gustavo [1 ,2 ]
Oulton, Rupert F. [3 ]
Bragas, Andrea V. [1 ,2 ]
Maier, Stefan A. [3 ]
机构
[1] Univ Buenos Aires, FCEN, Dept Fis, Lab Elect Cuant, Buenos Aires, DF, Argentina
[2] IFIBA CONICET, Buenos Aires, DF, Argentina
[3] Univ London Imperial Coll Sci Technol & Med, Dept Phys, Blackett Lab, London SW7 2AZ, England
来源
NATURE COMMUNICATIONS | 2015年 / 6卷
基金
英国工程与自然科学研究理事会;
关键词
SILICON NANOPARTICLES; FIELD ENHANCEMENT; LIGHT; GOLD; GENERATION; EFFICIENCY; SCATTERING; PLATFORM; HOTSPOTS;
D O I
10.1038/ncomms8915
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Nanoplasmonics has recently revolutionized our ability to control light on the nanoscale. Using metallic nanostructures with tailored shapes, it is possible to efficiently focus light into nanoscale field 'hot spots'. High field enhancement factors have been achieved in such optical nanoantennas, enabling transformative science in the areas of single molecule interactions, highly enhanced nonlinearities and nanoscale waveguiding. Unfortunately, these large enhancements come at the price of high optical losses due to absorption in the metal, severely limiting real-world applications. Via the realization of a novel nanophotonic platform based on dielectric nanostructures to form efficient nanoantennas with ultra-low light-into-heat conversion, here we demonstrate an approach that overcomes these limitations. We show that dimer-like silicon-based single nanoantennas produce both high surface enhanced fluorescence and surface enhanced Raman scattering, while at the same time generating a negligible temperature increase in their hot spots and surrounding environments.
引用
收藏
页数:8
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