Removal of nitric oxide in flue gases by multipoint to plane dielectric barrier discharge

被引:64
作者
Takaki, K [1 ]
Jani, MA [1 ]
Fujiwara, T [1 ]
机构
[1] Iwate Univ, Dept Elect & Elect Engn, Morioka, Iwate 0208551, Japan
基金
日本学术振兴会;
关键词
barrier discharge; chemical reaction; flue gas treatment; low temperature plasma; NOx; NOx reduction; silent discharge; streamer;
D O I
10.1109/27.782294
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
An experimental study on the removal of NO, in flue gas has been carried out using plasma chemical reactions in a dielectric barrier discharge. A multipoint-to-plane geometry is used for electrode to lower the operating voltage. The effect of the multipoint electrode configuration on the characteristics of a discharge and NO, removal has been investigated. Plasma is produced in a narrow gap by a dielectric barrier discharge at low applied voltage with sinusoidal waveform of 2-3 kV rms Specific energy to reduce NO is 63 eV. Electric energy consumed in the discharge increases linearly with area of multipoint electrode, and is approximately 1 mu J/point at 2.7 kV. In regard to the multipoint electrode configuration, the consumed energy can be increased by making angle of the point small. However, the energy efficiency of NO removal becomes small if the point angle is small. It also decreases with reducing the number of points per unit area. In regard to treatment of exhaust gas from a diesel engine generator (20 kVA), NO can be almost completely depleted by the multipoint-to-plane barrier discharge for electrical load below 35% of the rated output.
引用
收藏
页码:1137 / 1145
页数:9
相关论文
共 32 条
[21]  
KLEIN M, 1995, P 11 INT C GAS DISCH, V2, P414
[22]   THEORETICAL-ANALYSIS OF REMOVAL OF OXIDES OF SULFUR AND NITROGEN IN PULSED OPERATION OF ELECTROSTATIC PRECIPITATORS [J].
LOWKE, JJ ;
MORROW, R .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 1995, 23 (04) :661-671
[23]   NOVEL PLASMA CHEMICAL TECHNOLOGIES - PPCP AND SPCP FOR CONTROL OF GASEOUS-POLLUTANTS AND AIR TOXICS [J].
MASUDA, S ;
HOSOKAWA, S ;
TU, X ;
WANG, Z .
JOURNAL OF ELECTROSTATICS, 1995, 34 (04) :415-438
[24]   CONTROL OF NOX BY POSITIVE AND NEGATIVE PULSED CORONA DISCHARGES [J].
MASUDA, S ;
NAKAO, H .
IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, 1990, 26 (02) :374-383
[25]   Time dependence of NOx removal rate by a corona radical shower system [J].
Ohkubo, T ;
Kanazawa, S ;
Nomoto, Y ;
Chang, JS ;
Adachi, T .
IEEE TRANSACTIONS ON INDUSTRY APPLICATIONS, 1996, 32 (05) :1058-1062
[26]   ELECTRICAL CHARACTERISTICS OF A COAXIAL DIELECTRIC BARRIER DISCHARGE [J].
PASHAIE, B ;
DHALI, SK ;
HONEA, FI .
JOURNAL OF PHYSICS D-APPLIED PHYSICS, 1994, 27 (10) :2107-2110
[27]   TECHNIQUES FOR NONTHERMAL PLASMA PROCESSING OF NO IN N-2 [J].
PENETRANTE, BM ;
HSIAO, MC ;
MERRITT, BT ;
VOGTLIN, GE ;
WALLMAN, PH .
IEEE TRANSACTIONS ON PLASMA SCIENCE, 1995, 23 (04) :679-687
[28]   REDUCTION OF NITRIC-OXIDE IN FLUE-GASES BY POINT TO PLANE CORONA DISCHARGE WITH CATALYTIC COATINGS ON THE PLANE ELECTRODE [J].
SUHR, H ;
WEDDIGEN, G .
COMBUSTION SCIENCE AND TECHNOLOGY, 1990, 72 (1-3) :101-115
[29]   Non-thermal plasma remediation of SO2/NO using a dielectric-barrier discharge [J].
Sun, WM ;
Pashaie, B ;
Dhali, SK ;
Honea, FI .
JOURNAL OF APPLIED PHYSICS, 1996, 79 (07) :3438-3444
[30]  
Suzuki T., 1997, Transactions of the Institute of Electrical Engineers of Japan, Part A, V117-A, P1084