Surface and bulk components in angle-resolved core-level photoemission spectroscopy of graphite

被引:20
作者
Hunt, Michael R. C. [1 ]
机构
[1] Univ Durham, Dept Phys, Durham DH1 3LE, England
来源
PHYSICAL REVIEW B | 2008年 / 78卷 / 15期
基金
英国工程与自然科学研究理事会;
关键词
D O I
10.1103/PhysRevB.78.153408
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Angle-resolved x-ray photoelectron spectroscopy of the C 1s line of highly oriented pyrolytic graphite reveals two components separated by 194 +/- 6 meV, with markedly different asymmetry parameters and natural linewidth. Analysis of the intensity of these peaks as a function of angle demonstrates that the higher binding-energy peak is associated with the outermost graphite layer(s). The conflicting core-level photoemission data from graphite in the literature are addressed in light of these measurements.
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页数:4
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共 18 条
[1]  
Balasubramanian T, 2001, PHYS REV B, V64, DOI [10.1103/PhysRevB.64.205420, 10.1103/PhysRevLett.87.205420]
[2]   Photoemission study of onionlike carbons produced by annealing nanodiamonds [J].
Butenko, YV ;
Krishnamurthy, S ;
Chakraborty, AK ;
Klznetsov, VL ;
Dhanak, VR ;
Hunt, MRC ;
Siller, L .
PHYSICAL REVIEW B, 2005, 71 (07)
[3]   ANGLE-RESOLVED X-RAY-PHOTOELECTRON SPECTROSCOPY OF HIGHLY ORIENTED PYROLITIC GRAPHITE [J].
HOFFMAN, A ;
NYBERG, GL ;
LIESEGANG, J .
PHYSICAL REVIEW B, 1992, 45 (10) :5679-5682
[4]   Core level energy splitting in the C 1s photoelectron spectrum of C2H2 [J].
Kempgens, B ;
Koppel, H ;
Kivimaki, A ;
Neeb, M ;
Cederbaum, LS ;
Bradshaw, AM .
PHYSICAL REVIEW LETTERS, 1997, 79 (19) :3617-3620
[5]   Reentrant metallic behavior of graphite in the quantum limit [J].
Kopelevich, Y ;
Torres, JHS ;
da Silva, RR ;
Mrowka, F ;
Kempa, H ;
Esquinazi, P .
PHYSICAL REVIEW LETTERS, 2003, 90 (15) :4
[6]   C 1s photoemission spectrum in graphite(0001) [J].
Lizzit, S. ;
Petaccia, L. ;
Goldoni, A. ;
Larciprete, R. ;
Hofmann, Ph. ;
Zampieri, G. .
PHYSICAL REVIEW B, 2007, 76 (15)
[7]   Vibrational broadening of x-ray emission spectra: A first-principles study on diamond [J].
Mader, KA ;
Baroni, S .
PHYSICAL REVIEW B, 1997, 55 (15) :9649-9658
[8]   Core-level photoemission from graphite [J].
Prince, KC ;
Ulrych, I ;
Peloi, M ;
Ressel, B ;
Cháb, V ;
Crotti, C ;
Comicioli, C .
PHYSICAL REVIEW B, 2000, 62 (11) :6866-6868
[9]   LIFETIME AND SCREENING OF THE C1S PHOTOEMISSION IN GRAPHITE [J].
SETTE, F ;
WERTHEIM, GK ;
MA, Y ;
MEIGS, G ;
MODESTI, S ;
CHEN, CT .
PHYSICAL REVIEW B, 1990, 41 (14) :9766-9770
[10]   Ab initio calculation of graphite surface-bulk core-level splitting -: art. no. 073403 [J].
Simunek, A ;
Vackár, J .
PHYSICAL REVIEW B, 2004, 69 (07)