Synergistically enhanced electrochemical (ORR) activity of graphene oxide using boronic acid as an interlayer spacer

被引：25

作者：

Pourazadi, Ehsan ^{[1
]}

Haque, Enamul ^{[1
]}

Zhang, Weimin ^{[1
]}

Harris, Andrew T. ^{[1
]}

Minett, Andrew I. ^{[1
]}

机构：

[1] Univ Sydney, Fac Informat & Engn, Sch Chem & Biomol Engn, Lab Sustainable Technol, Sydney, NSW 2006, Australia

来源：

CHEMICAL COMMUNICATIONS | 2013年 / 49卷 / 94期

关键词：

OXYGEN REDUCTION REACTION; DOPED CARBON NANOTUBES; ELECTROCATALYSTS; CATALYSTS; METAL;

D O I：

10.1039/c3cc46741d

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Herein, boronic acid is incorporated into a graphene oxide (GO) structure in order to synthesise a graphene organic framework (GOF) with enhanced electrochemical performance. The results obtained indicate that the GOF favours a 4e(-) reduction pathway in the oxygen reduction reaction (ORR).

引用

收藏

页码：11068 / 11070

页数：3

相关论文

共 27 条

[1] Graphene Oxide Framework Materials: Theoretical Predictions and Experimental Results [J].

Burress, Jacob W. ;

Gadipelli, Srinivas ;

Ford, Jamie ;

Simmons, Jason M. ;

Zhou, Wei ;

Yildirim, Taner .

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION, 2010, 49 (47) :8902-8904

[2] Carbon-based Cathode Materials Doped with a New Borazine Compound for Electrochemical Oxygen Reduction [J].

Chang, Cha Wen ;

Nabae, Yuta ;

Kuroki, Shigeki ;

Hayakawa, Teruaki ;

Kakimoto, Masa-aki ;

Miyata, Seizo .

CHEMISTRY LETTERS, 2012, 41 (09) :923-925

[3] A Nitrogen-Doped Graphene/Carbon Nanotube Nanocomposite with Synergistically Enhanced Electrochemical Activity [J].

Chen, Ping ;

Xiao, Tian-Yuan ;

Qian, Yu-Hong ;

Li, Shan-Shan ;

Yu, Shu-Hong .

ADVANCED MATERIALS, 2013, 25 (23) :3192-3196

[4] Hydrothermal synthesis of macroscopic nitrogen-doped graphene hydrogels for ultrafast supercapacitor [J].

Chen, Ping ;

Yang, Jing-Jing ;

Li, Shan-Shan ;

Wang, Zheng ;

Xiao, Tian-Yuan ;

Qian, Yu-Hong ;

Yu, Shu-Hong .

NANO ENERGY, 2013, 2 (02) :249-256

[5] Oxygen reduction reaction on active sites of heteroatom-doped graphene [J].

Fan, Xiaofeng ;

Zheng, W. T. ;

Kuo, Jer-Lai .

RSC ADVANCES, 2013, 3 (16) :5498-5505

[6] Intercalation and stitching of graphite oxide with diaminoalkanes [J].

Herrera-Alonso, Margarita ;

Abdala, Ahmed A. ;

McAllister, Michael J. ;

Aksay, Ilhan A. ;

Prud'homme, Robert K. .

LANGMUIR, 2007, 23 (21) :10644-10649

[7] X-ray photoelectron spectroscopy investigation of boron carbide films deposited by sputtering [J].

Jacobsohn, LG ;

Schulze, RK ;

da Costa, MEHM ;

Nastasi, M .

SURFACE SCIENCE, 2004, 572 (2-3) :418-424

[8] A Graphene Oxide and Copper-Centered Metal Organic Framework Composite as a Tri-Functional Catalyst for HER, OER, and ORR [J].

Jahan, Maryam ;

Liu, Zhaolin ;

Loh, Kian Ping .

ADVANCED FUNCTIONAL MATERIALS, 2013, 23 (43) :5363-5372

[9] Structure of graphite oxide revisited [J].

Lerf, A ;

He, HY ;

Forster, M ;

Klinowski, J .

JOURNAL OF PHYSICAL CHEMISTRY B, 1998, 102 (23) :4477-4482

[10] Nitrogen-Doped Graphene Quantum Dots with Oxygen-Rich Functional Groups [J].

Li, Yan ;

Zhao, Yang ;

Cheng, Huhu ;

Hu, Yue ;

Shi, Gaoquan ;

Dai, Liming ;

Qu, Liangti .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2012, 134 (01) :15-18