共 48 条
Critical light instability in CB/DIO processed PBDTTT-EFT:PC71BM organic photovoltaic devices
被引:86
作者:

Pearson, Andrew J.
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Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England

Hopkinson, Paul E.
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Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England
Heidelberg Univ, Ctr Adv Mat, D-69120 Heidelberg, Germany
Heidelberg Univ, Kirchhoff Inst Phys, D-69120 Heidelberg, Germany Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England

Couderc, Elsa
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Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England

Domanski, Konrad
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Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England
Swiss Fed Inst Technol, Dept Chem & Chem Engn, Lab Photon & Interfaces, Stn 6, CH-1015 Lausanne, Switzerland Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England

Abdi-Jalebi, Mojtaba
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Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England

Greenham, Neil C.
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Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England
机构:
[1] Univ Cambridge, Cavendish Lab, JJ Thomson Ave, Cambridge CB3 0HE, England
[2] Heidelberg Univ, Ctr Adv Mat, D-69120 Heidelberg, Germany
[3] Heidelberg Univ, Kirchhoff Inst Phys, D-69120 Heidelberg, Germany
[4] Swiss Fed Inst Technol, Dept Chem & Chem Engn, Lab Photon & Interfaces, Stn 6, CH-1015 Lausanne, Switzerland
基金:
英国工程与自然科学研究理事会;
关键词:
PBDTTT-EFT;
PC71BM;
OPV;
Lifetime;
Solar;
Instability;
POLYMER SOLAR-CELLS;
OPEN-CIRCUIT VOLTAGE;
HIGH-PERFORMANCE;
EFFICIENCY;
MORPHOLOGY;
ADDITIVES;
RECOMBINATION;
OXYGEN;
LAYER;
D O I:
10.1016/j.orgel.2015.12.024
中图分类号:
T [工业技术];
学科分类号:
08 ;
摘要:
Organic photovoltaic (OPV) devices often undergo 'burn-in' during the early stages of operation, this period describing the relatively rapid drop in power output before stabilising. For normal and inverted PBDTTT-EFT:PC71BM OPVs prepared according to current protocols, we identify a critical and severe light-induced burn-in phase that reduces power conversion efficiency by at least 60% after 24 hours simulated AM1.5 illumination. Such losses result primarily from a reduction in photocurrent, and for inverted devices we correlate this process in-situ with the simultaneous emergence of space-chare effects on the ms timescale. The effects of burn in are also found to reduce the lifetime of photogenerated charge carriers, as determine by in-situ transient photovoltage measurements. To identify the underlying mechanisms of this instability, a range of techniques are employed ex-situ to separate bulk-and electrode-specific degradation processes. We find that whilst the active layer nanostructure and kinetics of free charge generation remain unchanged, partial photobleaching (6% of film O.D.) of PBDTTT-EFT:PC71BM occurs alongside an increase in the ground state bleach decay time of PBDTTT-EFT. We hypothesise that this latter observation may reflect relaxation from excited states on PBDTTT-EFT that do not undergo dissociation into free charges. Owing to the poor lifetime of the reference PBDTTT-EFT: PC71BM OPVs, the fabrication protocol is modified to identify routes for stability enhancement in this initially promising solar cell blend. (C) 2016 The Authors. Published by Elsevier B.V.
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页码:225 / 236
页数:12
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Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England

Lidzey, David G.
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Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England Univ Sheffield, Dept Phys & Astron, Sheffield S3 7RH, S Yorkshire, England
[40]
Morphological Stability and Performance of Polymer-Fullerene Solar Cells under Thermal Stress: The Impact of Photoinduced PC60BM Oligomerization
[J].
Wong, Him Cheng
;
Li, Zhe
;
Tan, Ching Hong
;
Zhong, Hongliang
;
Huang, Zhenggang
;
Bronstein, Hugo
;
McCulloch, Iain
;
Cabral, Joao T.
;
Durrant, James R.
.
ACS NANO,
2014, 8 (02)
:1297-1308

Wong, Him Cheng
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Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, Ctr Plast Elect, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, Ctr Plast Elect, London SW7 2AZ, England

Li, Zhe
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Univ London Imperial Coll Sci Technol & Med, Dept Chem, Ctr Plast Elect, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, Ctr Plast Elect, London SW7 2AZ, England

Tan, Ching Hong
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Univ London Imperial Coll Sci Technol & Med, Dept Chem, Ctr Plast Elect, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, Ctr Plast Elect, London SW7 2AZ, England

Zhong, Hongliang
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Univ London Imperial Coll Sci Technol & Med, Dept Chem, Ctr Plast Elect, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, Ctr Plast Elect, London SW7 2AZ, England

Huang, Zhenggang
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Univ London Imperial Coll Sci Technol & Med, Dept Chem, Ctr Plast Elect, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, Ctr Plast Elect, London SW7 2AZ, England

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McCulloch, Iain
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Univ London Imperial Coll Sci Technol & Med, Dept Chem, Ctr Plast Elect, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, Ctr Plast Elect, London SW7 2AZ, England

Cabral, Joao T.
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Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, Ctr Plast Elect, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, Ctr Plast Elect, London SW7 2AZ, England

Durrant, James R.
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Univ London Imperial Coll Sci Technol & Med, Dept Chem, Ctr Plast Elect, London SW7 2AZ, England Univ London Imperial Coll Sci Technol & Med, Dept Chem Engn, Ctr Plast Elect, London SW7 2AZ, England