A Selenophene-Based Low-Bandgap Donor-Acceptor Polymer Leading to Fast Ambipolar Logic

被引:309
作者
Kronemeijer, Auke J. [1 ]
Gili, Enrico [1 ]
Shahid, Munazza [2 ,3 ]
Rivnay, Jonathan [4 ]
Salleo, Alberto [4 ]
Heeney, Martin [2 ,3 ]
Sirringhaus, Henning [1 ]
机构
[1] Univ Cambridge, Cavendish Lab, Cambridge CB3 0HE, England
[2] Univ London Imperial Coll Sci Technol & Med, Dept Chem, London SW7 2AZ, England
[3] Univ London Imperial Coll Sci Technol & Med, Ctr Plast Elect, London SW7 2AZ, England
[4] Stanford Univ, Dept Mat Sci & Engn, Stanford, CA 94305 USA
基金
英国工程与自然科学研究理事会;
关键词
organic electronics; field-effect transistors; selenophene; polymer semiconductor; ambipolar logic; FIELD-EFFECT TRANSISTORS; HIGH-PERFORMANCE; MOLECULAR PACKING; CHARGE-TRANSPORT; MOBILITY; COPOLYMER; CIRCUITS; ELECTRON; HOLE;
D O I
10.1002/adma.201104522
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Fast ambipolar CMOS-like logic is demonstrated using a new selenophene-based donor-acceptor polymer semiconductor. The polymer exhibits saturation hole and electron mobilities of 0.46 cm 2/Vs and 0.84 cm 2/Vs. Inverters are fabricated with high gains while three-stage ring oscillators show stable oscillation with an unprecedented maximum frequency of 182 kHz at a relatively low supply voltage of 50 V. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.
引用
收藏
页码:1558 / 1565
页数:8
相关论文
共 43 条
[1]   Synthesis, Characterization, and Field Effect Transistor Properties of Regioregular Poly(3-alkyl-2,5-selenylenevinylene) [J].
Al-Hashimi, Mohammed ;
Baklar, Mohammed A. ;
Colleaux, Florian ;
Watkins, Scott E. ;
Anthopoulos, Thomas D. ;
Stingelin, Natalie ;
Heeney, Martin .
MACROMOLECULES, 2011, 44 (13) :5194-5199
[2]   Air-stable complementary-like circuits based on organic ambipolar transistors [J].
Anthopoulos, Thomas D. ;
Setayesh, Sepas ;
Smits, Edsger ;
Colle, Michael ;
Cantatore, Eugenio ;
de Boer, Bert ;
Blom, Paul W. M. ;
de Leeuw, Dago M. .
ADVANCED MATERIALS, 2006, 18 (14) :1900-+
[3]   Silaindacenodithiophene Semiconducting Polymers for Efficient Solar Cells and High-Mobility Ambipolar Transistors [J].
Ashraf, Raja Shahid ;
Chen, Zhuoying ;
Leem, Dong Seok ;
Bronstein, Hugo ;
Zhang, Weimin ;
Schroeder, Bob ;
Geerts, Yves ;
Smith, Jeremy ;
Watkins, Scott ;
Anthopoulos, Thomas D. ;
Sirringhaus, Henning ;
de Mello, John C. ;
Heeney, Martin ;
McCulloch, Iain .
CHEMISTRY OF MATERIALS, 2011, 23 (03) :768-770
[4]   Charge Injection Engineering of Ambipolar Field-Effect Transistors for High-Performance Organic Complementary Circuits [J].
Baeg, Kang-Jun ;
Kim, Juhwan ;
Khim, Dongyoon ;
Caironi, Mario ;
Kim, Dong-Yu ;
You, In-Kyu ;
Quinn, Jordan R. ;
Facchetti, Antonio ;
Noh, Yong-Young .
ACS APPLIED MATERIALS & INTERFACES, 2011, 3 (08) :3205-3214
[5]   Improved performance uniformity of inkjet printed n-channel organic field-effect transistors and complementary inverters [J].
Baeg, Kang-Jun ;
Khim, Dongyoon ;
Kim, Ju-Hwan ;
Kang, Minji ;
You, In-Kyu ;
Kim, Dong-Yu ;
Noh, Yong-Young .
ORGANIC ELECTRONICS, 2011, 12 (04) :634-640
[6]   High Speeds Complementary Integrated Circuits Fabricated with All-Printed Polymeric Semiconductors [J].
Baeg, Kang-Jun ;
Khim, Dongyoon ;
Kim, Dong-Yu ;
Jung, Soon-Won ;
Koo, Jae Bon ;
You, In-Kyu ;
Yan, Henry ;
Facchetti, Antonio ;
Noh, Yong-Young .
JOURNAL OF POLYMER SCIENCE PART B-POLYMER PHYSICS, 2011, 49 (01) :62-67
[7]   Poly(diketopyrrolopyrrole-terthiophene) for Ambipolar Logic and Photovoltaics [J].
Bijleveld, Johan C. ;
Zoombelt, Arjan P. ;
Mathijssen, Simon G. J. ;
Wienk, Martijn M. ;
Turbiez, Mathieu ;
de Leeuw, Dago M. ;
Janssen, Rene A. J. .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (46) :16616-+
[8]   Thieno[3,2-b]thiophene-Diketopyrrolopyrrole-Containing Polymers for High-Performance Organic Field-Effect Transistors and Organic Photovoltaic Devices [J].
Bronstein, Hugo ;
Chen, Zhuoying ;
Ashraf, Rap Shahid ;
Zhang, Weimin ;
Du, Junping ;
Durrant, James R. ;
Tuladhar, Pabitra Shakya ;
Song, Kigook ;
Watkins, Scott E. ;
Geerts, Yves ;
Wienk, Martijn M. ;
Janssen, Rene A. J. ;
Anthopoulos, Thomas ;
Sirringhaus, Henning ;
Heeney, Martin ;
McCulloch, Iain .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (10) :3272-3275
[9]   High-mobility ambipolar near-infrared light-emitting polymer field-effect transistors [J].
Buergi, Lukas ;
Turbiez, Mathieu ;
Pfeiffer, Reto ;
Bienewald, Frank ;
Kirner, Hans-Joerg ;
Winnewisser, Carsten .
ADVANCED MATERIALS, 2008, 20 (11) :2217-2224
[10]   High-Performance Ambipolar Diketopyrrolopyrrole-Thieno[3,2-b]thiophene Copolymer Field-Effect Transistors with Balanced Hole and Electron Mobilities [J].
Chen, Zhuoying ;
Lee, Mi Jung ;
Ashraf, Raja Shahid ;
Gu, Yun ;
Albert-Seifried, Sebastian ;
Nielsen, Martin Meedom ;
Schroeder, Bob ;
Anthopoulos, Thomas D. ;
Heeney, Martin ;
McCulloch, Iain ;
Sirringhaus, Henning .
ADVANCED MATERIALS, 2012, 24 (05) :647-+