Molecular and textural engineering of conjugated carbon nitride catalysts for selective oxidation of alcohols with visible light

被引:173
作者
Chen, Yan [1 ]
Zhang, Jinshui [1 ]
Zhang, Mingwen [1 ]
Wang, Xinchen [1 ]
机构
[1] Fuzhou Univ, Res Inst Photocatalysis, Coll Chem & Chem Engn, Fujian Prov Key Lab Photocatalysis,State Key Lab, Fuzhou 350002, Peoples R China
基金
中国国家自然科学基金;
关键词
METAL-FREE ACTIVATION; HYDROGEN EVOLUTION; AEROBIC OXIDATION; ALDEHYDES; SEMICONDUCTORS; IRRADIATION; G-C3N4; OXYGEN; O-2;
D O I
10.1039/c3sc51203g
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A thiophene motif has been integrated into mesoporous carbon nitride (MCN) to improve the photoactivation of molecular oxygen towards the selective oxidation of alcohols. This modification also extends the photoactive part of the spectrum of MCN by electronic modification of the conjugated system.
引用
收藏
页码:3244 / 3248
页数:5
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