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Adsorptive removal of hazardous materials using metal-organic frameworks (MOFs): A review

被引：1181
作者：
Khan, Nazmul Abedin
Hasan, Zubair
Jhung, Sung Hwa [1 ]
机构：
[1] Kyungpook Natl Univ, Dept Chem, Taegu 702701, South Korea
来源：
JOURNAL OF HAZARDOUS MATERIALS | 2013年 / 244卷
基金：
新加坡国家研究基金会;
关键词：
Adsorption; Adsorptive removal; Hazardous materials; Metal-organic frameworks; Review; CARBON-DIOXIDE CAPTURE; LIQUID-PHASE ADSORPTION; SCIENCE-AND-TECHNOLOGY; ACTIVATED CARBON; HEAVY-METAL; CO2; ADSORPTION; HIGH-CAPACITY; ION-EXCHANGE; JET FUEL; COORDINATION POLYMERS;
D O I：
10.1016/j.jhazmat.2012.11.011
中图分类号：
X [环境科学、安全科学];
学科分类号：
08 ; 0830 ;
摘要：
Efficient removal of hazardous materials from the environment has become an important issue from a biological and environmental standpoint. Adsorptive removal of toxic components from fuel, wastewater or air is one of the most attractive approaches for cleaning technologies. Recently, porous metal-organic framework (MOF) materials have been very promising in the adsorption/separation of various liquids and gases due to their unique characteristics. This review summarizes the recent literatures on the adsorptive removal of various hazardous compounds mainly from fuel, water, and air by virgin or modified MOF materials. Possible interactions between the adsorbates and active adsorption sites of the MOFs will be also discussed to understand the adsorption mechanism. Most of the observed results can be explained with the following mechanisms: (1) adsorption onto a coordinatively unsaturated site, (2) adsorption via acid-base interaction, (3) adsorption via pi-complex formation, (4) adsorption via hydrogen bonding, (5) adsorption via electrostatic interaction, and (6) adsorption based on the breathing properties of some MOFs and so on. (c) 2012 Elsevier B.V. All rights reserved.
引用
收藏
页码：444 / 456
页数：13
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