Single-molecule vibrational spectroscopy and microscopy: CO on Cu(001) and Cu(110)

被引:134
作者
Lauhon, LJ [1 ]
Ho, W
机构
[1] Cornell Univ, Atom & Solid State Phys Lab, Ithaca, NY 14853 USA
[2] Cornell Univ, Ctr Mat Res, Ithaca, NY 14853 USA
来源
PHYSICAL REVIEW B | 1999年 / 60卷 / 12期
关键词
D O I
10.1103/PhysRevB.60.R8525
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Single-molecule vibrations of four isotopes of CO on Cu(001) and Cu(110) at 8 K have been measured by inelastic electron tunneling spectroscopy with the scanning tunneling microscope (STM-IETS). While the low energy hindered rotation exhibits strong intensity, the C-O stretch approaches the present detection limit of STM-IETS. By performing vibrational microscopy, the spatial distribution of the hindered rotation intensity is found to be more localized than the topographic depression in constant current images. [S0163-1829(99)50336-6].
引用
收藏
页码:R8525 / R8528
页数:4
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