Initial oxidation processes of H-terminated Si(100) surfaces analyzed using a random sequential adsorption model

被引:8
作者
Ikeda, H
Nakagawa, Y
Zaima, S
Ishibashi, Y
Yasuda, Y
机构
[1] Nagoya Univ, Grad Sch Engn, Dept Crystalline Mat Sci, Chikusa Ku, Nagoya, Aichi 4648603, Japan
[2] Nagoya Univ, Ctr Cooperat Res Adv Sci & Technol, Chikusa Ku, Nagoya, Aichi 4648603, Japan
[3] Nagoya Univ, Grad Sch Engn, Dept Appl Phys, Chikusa Ku, Nagoya, Aichi 4648603, Japan
来源
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS BRIEF COMMUNICATIONS & REVIEW PAPERS | 1999年 / 38卷 / 6A期
关键词
initial oxidation process; H-terminated Si(100) surface; random sequential adsorption model; HREELS; sticking probability;
D O I
10.1143/JJAP.38.3422
中图分类号
O59 [应用物理学];
学科分类号
摘要
We have applied a random sequential adsorption (RSA) model to the experimental results of the adsorption of O atom's on a H-terminated Si(100) surface and discussed the initial oxidation processes on H-terminated Si(100)-1 x 1 surfaces. The RSA model can reproduce the experimental results obtained by high-resolution electron energy loss spectroscopy (HREELS) and clearly indicates that O atoms preferentially adsorb on one of two back-bond sites of a surface Si atom. In addition, it is also indicated that the adsorption of O atoms on Si-Si bonds between the second- and third-layer Si atoms from the surface hardly occurs until all back-bond sites of surface Si atoms are occupied by O atoms.
引用
收藏
页码:3422 / 3425
页数:4
相关论文
共 15 条
[1]   QUASIEQUILIBRIUM TREATMENT OF GAS-SOLID REACTIONS .I. EVAPORATION RATES OF VOLATILE SPECIES FORMED IN REACTION OF O2 WITH W, MO, AND C [J].
BATTY, JC ;
STICKNEY, RE .
JOURNAL OF CHEMICAL PHYSICS, 1969, 51 (10) :4475-&
[2]   REACTIVE ATOM SURFACE SCATTERING - THE ADSORPTION AND REACTION OF ATOMIC OXYGEN ON THE SI(100) SURFACE [J].
ENGSTROM, JR ;
NELSON, MM ;
ENGEL, T .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A-VACUUM SURFACES AND FILMS, 1989, 7 (03) :1837-1840
[3]   ADSORPTION STATES AND ADSORPTION-KINETICS OF ATOMIC-HYDROGEN ON SILICON CRYSTAL-SURFACES [J].
FROITZHEIM, H ;
KOHLER, U ;
LAMMERING, H .
SURFACE SCIENCE, 1985, 149 (2-3) :537-557
[4]   COOPERATIVE EFFECTS IN RANDOM SEQUENTIAL POLYMER REACTIONS [J].
GONZALEZ, JJ ;
HEMMER, PC ;
HOYE, JS .
CHEMICAL PHYSICS, 1974, 3 (02) :228-238
[5]   IDEAL HYDROGEN TERMINATION OF THE SI-(111) SURFACE [J].
HIGASHI, GS ;
CHABAL, YJ ;
TRUCKS, GW ;
RAGHAVACHARI, K .
APPLIED PHYSICS LETTERS, 1990, 56 (07) :656-658
[6]   EFFECTS OF SURFACE HYDROGEN ON THE AIR OXIDATION AT ROOM-TEMPERATURE OF HF-TREATED SI(100) SURFACES [J].
HIRASHITA, N ;
KINOSHITA, M ;
AIKAWA, I ;
AJIOKA, T .
APPLIED PHYSICS LETTERS, 1990, 56 (05) :451-453
[7]   Initial oxidation processes of H-terminated Si(100) surfaces studied by high-resolution electron energy loss spectroscopy [J].
Ikeda, H ;
Hotta, K ;
Furuta, S ;
Zaima, S ;
Yasuda, Y .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS SHORT NOTES & REVIEW PAPERS, 1996, 35 (2B) :1069-1072
[8]   Influences of hydrogen on initial oxidation processes of H-terminated Si(100) surfaces [J].
Ikeda, H ;
Hotta, K ;
Furuta, S ;
Zaima, S ;
Yasuda, Y .
APPLIED SURFACE SCIENCE, 1996, 104 :354-358
[9]   OXIDATION OF H-TERMINATED SI(100) SURFACES STUDIED BY HIGH-RESOLUTION ELECTRON-ENERGY-LOSS SPECTROSCOPY [J].
IKEDA, H ;
HOTTA, K ;
YAMADA, T ;
ZAIMA, S ;
IWANO, H ;
YASUDA, Y .
JOURNAL OF APPLIED PHYSICS, 1995, 77 (10) :5125-5129
[10]  
IKEDA H, IN PRESS JPN J APPL