Effect of Selenophene in a DPP Copolymer Incorporating a Vinyl Group for High-Performance Organic Field-Effect Transistors

被引：239

作者：

Kang, Il ^{[1
]}

An, Tae Kyu ^{[4
]}

Hong, Jung-a ^{[1
]}

Yun, Hui-Jun ^{[1
]}

Kim, Ran ^{[2
,3
]}

Chung, Dae Sung ^{[5
]}

Park, Chan Eon ^{[4
]}

Kim, Yun-Hi ^{[2
,3
]}

Kwon, Soon-Ki ^{[1
]}

机构：

[1] Gyeongsang Natl Univ, Res Inst Green Energy Convergence Technol REGET, Sch Mat Sci & Engn, Jinju 660701, South Korea

[2] Gyeongsang Natl Univ, Dept Chem, Jinju 660701, South Korea

[3] RINS, Jinju 660701, South Korea

[4] Pohang Univ Sci & Technol, Dept Chem Engn, Organ Elect Lab, Pohang 790784, South Korea

[5] Dong A Univ, Dept Chem Engn, Pusan 604714, South Korea

来源：

ADVANCED MATERIALS | 2013年 / 25卷 / 04期

基金：

新加坡国家研究基金会;

关键词：

conjugated polymer; donor-acceptor systems; organic thin-film transistors; p-channel organic semiconductors; selenophene; 1; 4-diketopyrrolo[3; 4-c]pyrrole; THIN-FILM TRANSISTORS; END-CAPPED OLIGOMERS; HIGH-MOBILITY; CONJUGATED POLYMERS; SIDE-CHAINS; SOLAR-CELLS; AMBIPOLAR; ACCEPTOR; DIKETOPYRROLOPYRROLE; DONOR;

D O I：

10.1002/adma.201202867

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A new polymeric semiconductor, PDPPDTSE, is reported which is composed of a diketopyrrolopyrrole moiety and selenophenylene vinylene selenophene, with a high field-effect mobility achieved through intermolecular donor-acceptor interactions. The field-effect mobility of OFET devices based on PDPPDTSE by spin-casting is 4.97 cm(2) V-1 s(-1), which is higher than predecessor polymeric semiconductors.

引用

收藏

页码：524 / 528

页数：5

相关论文

共 41 条

[1] Poly(diketopyrrolopyrrole-terthiophene) for Ambipolar Logic and Photovoltaics [J].

Bijleveld, Johan C. ;

Zoombelt, Arjan P. ;

Mathijssen, Simon G. J. ;

Wienk, Martijn M. ;

Turbiez, Mathieu ;

de Leeuw, Dago M. ;

Janssen, Rene A. J. .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (46) :16616-+

[2] Thieno[3,2-b]thiophene-Diketopyrrolopyrrole-Containing Polymers for High-Performance Organic Field-Effect Transistors and Organic Photovoltaic Devices [J].

Bronstein, Hugo ;

Chen, Zhuoying ;

Ashraf, Rap Shahid ;

Zhang, Weimin ;

Du, Junping ;

Durrant, James R. ;

Tuladhar, Pabitra Shakya ;

Song, Kigook ;

Watkins, Scott E. ;

Geerts, Yves ;

Wienk, Martijn M. ;

Janssen, Rene A. J. ;

Anthopoulos, Thomas ;

Sirringhaus, Henning ;

Heeney, Martin ;

McCulloch, Iain .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (10) :3272-3275

[3] High-mobility ambipolar near-infrared light-emitting polymer field-effect transistors [J].

Buergi, Lukas ;

Turbiez, Mathieu ;

Pfeiffer, Reto ;

Bienewald, Frank ;

Kirner, Hans-Joerg ;

Winnewisser, Carsten .

ADVANCED MATERIALS, 2008, 20 (11) :2217-2224

[4] Highly p-Extended Copolymers with Diketopyrrolopyrrole Moieties for High-Performance Field-Effect Transistors [J].

Chen, Huajie ;

Guo, Yunlong ;

Yu, Gui ;

Zhao, Yan ;

Zhang, Ji ;

Gao, Dong ;

Liu, Hongtao ;

Liu, Yunqi .

ADVANCED MATERIALS, 2012, 24 (34) :4618-4622

[5] High mobility organic single crystal transistors based on soluble triisopropylsilylethynyl anthracene derivatives [J].

Chung, Dae Sung ;

Park, Jong Won ;

Park, Jong-Hwa ;

Moon, Dohyun ;

Kim, Ghyung Hwa ;

Lee, Heung-Soo ;

Lee, Dong Hoon ;

Shim, Hong-Ku ;

Kwon, Soon-Ki ;

Park, Chan Eon .

JOURNAL OF MATERIALS CHEMISTRY, 2010, 20 (03) :524-530

[6] Alternating Copolymers Containing Bithiophene and Dialkoxynaphthalene for the Applications to Field Effect Transistor and Photovoltaic Cell: Performance and Stability [J].

Chung, Dae Sung ;

Park, Jong Won ;

Kim, Seul-Ong ;

Heo, Kyuyoung ;

Park, Chan Eon ;

Ree, Moonhor ;

Kim, Yun-Hi ;

Kwon, Soon-Ki .

CHEMISTRY OF MATERIALS, 2009, 21 (22) :5499-5507

[7]

Dou LT, 2012, NAT PHOTONICS, V6, P180, DOI [10.1038/nphoton.2011.356, 10.1038/NPHOTON.2011.356]

[8] The path to ubiquitous and low-cost organic electronic appliances on plastic [J].

Forrest, SR .

NATURE, 2004, 428 (6986) :911-918

[9] Selenophene-Thiophene Block Copolymer Solar Cells with Thermostable Nanostructures [J].

Gao, Dong ;

Hollinger, Jon ;

Seferos, Dwight S. .

ACS NANO, 2012, 6 (08) :7114-7121

[10] Thieno[3,4-c]pyrrole-4,6-dione-Based Polymer Semiconductors: Toward High-Performance, Air-Stable Organic Thin-Film Transistors [J].

Guo, Xugang ;

Ponce Ortiz, Rocio ;

Zheng, Yan ;

Kim, Myung-Gil ;

Zhang, Shiming ;

Hu, Yan ;

Lu, Gang ;

Facchetti, Antonio ;

Marks, Tobin J. .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (34) :13685-13697

← 1 2 3 4 5 →