Efficient Small Bandgap Polymer Solar Cells with High Fill Factors for 300 nm Thick Films

被引：294

作者：

Li, Weiwei ^{[1
]}

Hendriks, Koen H. ^{[1
]}

Roelofs, W. S. Christian ^{[1
]}

Kim, Youngju ^{[1
]}

Wienk, Martijn M. ^{[1
]}

Janssen, Rene A. J. ^{[1
]}

机构：

[1] Eindhoven Univ Technol, NL-5600 MB Eindhoven, Netherlands

来源：

ADVANCED MATERIALS | 2013年 / 25卷 / 23期

关键词：

conjugated polymers; organic electronics; organic solar cells; HIGH-PERFORMANCE AMBIPOLAR; FIELD-EFFECT TRANSISTORS; TANDEM POLYMER; GAP POLYMERS; FABRICATION;

D O I：

10.1002/adma.201300017

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A high-molecular-weight conjugated polymer based on alternating electron-rich and electron-deficient fused ring systems provides efficient polymer solar cells when blended with C-60 and C-70 fullerene derivatives. The morphology of the new polymer/fullerene blend reduces bimolecular recombination and allows reaching high fill factors and power conversion efficiencies for films up to 300 nm thickness.

引用

页码：3182 / 3186

页数：5

共 32 条

[1] Copolymers of diketopyrrolopyrrole and thienothiophene for photovoltaic cells [J].

Bijleveld, Johan C. ;

Verstrijden, R. A. Melanie ;

Wienk, Martijn M. ;

Janssen, Rene A. J. .

JOURNAL OF MATERIALS CHEMISTRY, 2011, 21 (25) :9224-9231

[2] Efficient Solar Cells Based on an Easily Accessible Diketopyrrolopyrrole Polymer [J].

Bijleveld, Johan C. ;

Gevaerts, Veronique S. ;

Di Nuzzo, Daniele ;

Turbiez, Mathieu ;

Mathijssen, Simon G. J. ;

de Leeuw, Dago M. ;

Wienk, Martijn M. ;

Janssen, Rene A. J. .

ADVANCED MATERIALS, 2010, 22 (35) :E242-+

[3] Poly(diketopyrrolopyrrole-terthiophene) for Ambipolar Logic and Photovoltaics [J].

Bijleveld, Johan C. ;

Zoombelt, Arjan P. ;

Mathijssen, Simon G. J. ;

Wienk, Martijn M. ;

Turbiez, Mathieu ;

de Leeuw, Dago M. ;

Janssen, Rene A. J. .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2009, 131 (46) :16616-+

[4] Device physics of polymer:fullerene bulk heterojunction solar cells [J].

Blom, Paul W. M. ;

Mihailetchi, Valentin D. ;

Koster, L. Jan Anton ;

Markov, Denis E. .

ADVANCED MATERIALS, 2007, 19 (12) :1551-1566

[5] Thieno[3,2-b]thiophene-Diketopyrrolopyrrole-Containing Polymers for High-Performance Organic Field-Effect Transistors and Organic Photovoltaic Devices [J].

Bronstein, Hugo ;

Chen, Zhuoying ;

Ashraf, Rap Shahid ;

Zhang, Weimin ;

Du, Junping ;

Durrant, James R. ;

Tuladhar, Pabitra Shakya ;

Song, Kigook ;

Watkins, Scott E. ;

Geerts, Yves ;

Wienk, Martijn M. ;

Janssen, Rene A. J. ;

Anthopoulos, Thomas ;

Sirringhaus, Henning ;

Heeney, Martin ;

McCulloch, Iain .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (10) :3272-3275

[6] Crystalline conjugated polymer containing fused 2,5-di(thiophen-2-yl)thieno[2,3-b]thiophene and thieno[3,4-c]pyrrole-4,6-dione units for bulk heterojunction solar cells [J].

Chen, Guan-Yu ;

Cheng, Yu-Hsin ;

Chou, Yi-Jen ;

Su, Ming-Shin ;

Chen, Chia-Min ;

Wei, Kung-Hwa .

CHEMICAL COMMUNICATIONS, 2011, 47 (17) :5064-5066

[7] High-Performance Ambipolar Diketopyrrolopyrrole-Thieno[3,2-b]thiophene Copolymer Field-Effect Transistors with Balanced Hole and Electron Mobilities [J].

Chen, Zhuoying ;

Lee, Mi Jung ;

Ashraf, Raja Shahid ;

Gu, Yun ;

Albert-Seifried, Sebastian ;

Nielsen, Martin Meedom ;

Schroeder, Bob ;

Anthopoulos, Thomas D. ;

Heeney, Martin ;

McCulloch, Iain ;

Sirringhaus, Henning .

ADVANCED MATERIALS, 2012, 24 (05) :647-+

[8] Bulk Heterojunction Solar Cells Using Thieno[3,4-c]pyrrole-4,6-dione and Dithieno[3,2-b:2′,3′-d]silole Copolymer with a Power Conversion Efficiency of 7.3% [J].

Chu, Ta-Ya ;

Lu, Jianping ;

Beaupre, Serge ;

Zhang, Yanguang ;

Pouliot, Jean-Remi ;

Wakim, Salem ;

Zhou, Jiayun ;

Leclerc, Mario ;

Li, Zhao ;

Ding, Jianfu ;

Tao, Ye .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2011, 133 (12) :4250-4253

[9]

Coffin RC, 2009, NAT CHEM, V1, P657, DOI [10.1038/NCHEM.403, 10.1038/nchem.403]

[10] Systematic Investigation of Benzodithiophene- and Diketopyrrolopyrrole-Based Low-Bandgap Polymers Designed for Single Junction and Tandem Polymer Solar Cells [J].

Dou, Letian ;

Gao, Jing ;

Richard, Eric ;

You, Jingbi ;

Chen, Chun-Chao ;

Cha, Kitty C. ;

He, Youjun ;

Li, Gang ;

Yang, Yang .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2012, 134 (24) :10071-10079

← 1 2 3 4 →