Direct observation of reaction-limited aggregation on semiconductor surfaces

被引:54
作者
Chang, TC [1 ]
Hwang, IS
Tsong, TT
机构
[1] Acad Sinica, Inst Phys, Taipei, Taiwan
[2] Natl Taiwan Univ, Dept Elect Engn, Taipei 10764, Taiwan
[3] Natl Taiwan Univ, Dept Phys, Taipei 10764, Taiwan
关键词
D O I
10.1103/PhysRevLett.83.1191
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report a discovery that the nucleation and growth of two-dimensional (2D) Ge islands at a Pb layer covered Si(111) surface are reaction limited. Using scanning tunneling microscopy, a compact-to-fractal island shape transition is observed as the; deposition flux is lowered, the temperature is raised, or at a low Ge coverage. This behavior is completely opposite to what was predicted from those theories based on diffusion-limited aggregation and previous experimental observations. Energy barriers are found to exist for the nucleation and growth of Ge islands, indicating that their growth behavior is exchange-reaction rate limited.
引用
收藏
页码:1191 / 1194
页数:4
相关论文
共 25 条
[1]  
Brune H, 1998, SURF SCI REP, V31, P121, DOI 10.1016/S0167-5729(99)80001-6
[2]   SURFACTANTS IN EPITAXIAL-GROWTH [J].
COPEL, M ;
REUTER, MC ;
KAXIRAS, E ;
TROMP, RM .
PHYSICAL REVIEW LETTERS, 1989, 63 (06) :632-635
[3]   THE ROLE OF ADSORBED GASES IN METAL ON METAL EPITAXY [J].
EGELHOFF, WF ;
STEIGERWALD, DA .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A-VACUUM SURFACES AND FILMS, 1989, 7 (03) :2167-2173
[4]   NUCLEATION AND GROWTH IN METAL-ON-METAL HOMOEPITAXY - RATE-EQUATIONS, SIMULATIONS AND EXPERIMENTS [J].
EVANS, JW ;
BARTELT, MC .
JOURNAL OF VACUUM SCIENCE & TECHNOLOGY A-VACUUM SURFACES AND FILMS, 1994, 12 (04) :1800-1808
[5]   GROWTH AND MORPHOLOGY OF PB ON SI(111) [J].
GANZ, E ;
HWANG, IS ;
XIONG, FL ;
THEISS, SK ;
GOLOVCHENKO, J .
SURFACE SCIENCE, 1991, 257 (1-3) :259-273
[6]   Atomic processes in low temperature Pt-dendrite growth on Pt(III) [J].
Hohage, M ;
Bott, M ;
Morgenstern, M ;
Zhang, ZY ;
Michely, T ;
Comsa, G .
PHYSICAL REVIEW LETTERS, 1996, 76 (13) :2366-2369
[7]   Growth mechanism and morphology of Ge on Pb covered Si(111)surfaces [J].
Hwang, IS ;
Chang, TC ;
Tsong, TT .
SURFACE SCIENCE, 1998, 410 (2-3) :L741-L747
[8]   Exchange-barrier effects on nucleation and growth of surfactant-mediated epitaxy [J].
Hwang, IS ;
Chang, TC ;
Tsong, TT .
PHYSICAL REVIEW LETTERS, 1998, 80 (19) :4229-4232
[9]   HIGH COVERAGE PHASES OF PB ON THE SI(111) SURFACE - STRUCTURES AND PHASE-TRANSITIONS [J].
HWANG, IS ;
MARTINEZ, RE ;
LIU, C ;
GOLOVCHENKO, JA .
SURFACE SCIENCE, 1995, 323 (03) :241-257
[10]   FRACTAL GROWTH OF 2-DIMENSIONAL ISLANDS - AU ON RU(0001) [J].
HWANG, RQ ;
SCHRODER, J ;
GUNTHER, C ;
BEHM, RJ .
PHYSICAL REVIEW LETTERS, 1991, 67 (23) :3279-3282