Low temperature magnetization of the S=1/2 kagome antiferromagnet ZnCu3(OH)6Cl2

被引:116
作者
Bert, F. [1 ]
Nakamae, S. [2 ]
Ladieu, F. [2 ]
L'Hote, D. [2 ]
Bonville, P. [2 ]
Duc, F.
Trombe, J. -C. [3 ]
Mendels, P. [1 ]
机构
[1] Univ Paris 11, CNRS, UMR 8502, Phys Solides Lab, F-91405 Orsay, France
[2] CEA Saclay, DSM, Serv Phys Etat Condense, F-91191 Gif Sur Yvette, France
[3] CNRS, UPR 8011, Ctr Elaborat Mat & Etudes Struct, F-31055 Toulouse, France
关键词
D O I
10.1103/PhysRevB.76.132411
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The dc magnetization of the unique S=1/2 kagome antiferromagnet Herbertsmithite has been measured down to 0.1 K. No sign of spin freezing is observed in agreement with former mu SR and ac-susceptibility results. The low temperature magnetic response is dominated by a defect contribution which exhibits an energy scale similar or equal to 1 K, likely reflecting the coupling of the defects. The defect component is saturated at low temperature by H greater than or similar to 8 T applied magnetic fields which enables us to estimate an upper bound for the nonsaturated intrinsic kagome susceptibility at T=1.7 K.
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页数:4
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共 23 条
[11]   Order versus disorder in the quantum Heisenberg antiferromagnet on the kagome lattice using exact spectra analysis [J].
Lecheminant, P ;
Bernu, B ;
Lhuillier, C ;
Pierre, L ;
Sindzingre, P .
PHYSICAL REVIEW B, 1997, 56 (05) :2521-2529
[12]   Quantum-spin-liquid states in the two-dimensional kagome antiferromagnets ZnxCu4-x(OD)6Cl2 [J].
Lee, S.-H. ;
Kikuchi, H. ;
Qiu, Y. ;
Lake, B. ;
Huang, Q. ;
Habicht, K. ;
Kiefer, K. .
NATURE MATERIALS, 2007, 6 (11) :853-857
[13]   Quantum magnetism in the paratacamite family: Towards an ideal kagome lattice [J].
Mendels, P. ;
Bert, F. ;
de Vries, M. A. ;
Olariu, A. ;
Harrison, A. ;
Duc, F. ;
Trombe, J. C. ;
Lord, J. S. ;
Amato, A. ;
Baines, C. .
PHYSICAL REVIEW LETTERS, 2007, 98 (07)
[14]   Ga NMR study of the local susceptibility in kagome-based SrCr8Ga4O19:: Pseudogap and paramagnetic defects [J].
Mendels, P ;
Keren, A ;
Limot, L ;
Mekata, M ;
Collin, G ;
Horvatic, M .
PHYSICAL REVIEW LETTERS, 2000, 85 (16) :3496-3499
[15]  
MISGUICH G, IN PRESS EUR PHYS J
[16]  
MISGUICH G, 2005, FRUSTRATION 2 DIMENS
[17]   Polarized neutron scattering study of the kagome antiferromagnet SrCr8Ga4O19 [J].
Mondelli, C ;
Andersen, K ;
Mutka, H ;
Payen, C ;
Frick, B .
PHYSICA B-CONDENSED MATTER, 1999, 267 :139-141
[18]  
OFER O, ARXIVCONDMAT0610540
[19]   Entropy balance and evidence for local spin singlets in a Kagome-like magnet [J].
Ramirez, AP ;
Hessen, B ;
Winklemann, M .
PHYSICAL REVIEW LETTERS, 2000, 84 (13) :2957-2960
[20]   Magnetic susceptibility of the Kagome antiferromagnet ZnCu3(OH)6Cl2 [J].
Rigol, Marcos ;
Singh, Rajiv R. P. .
PHYSICAL REVIEW LETTERS, 2007, 98 (20)