Surface-related emission in highly luminescent CdSe quantum dots

被引:498
作者
Wang, XY
Qu, LH
Zhang, JY
Peng, XG
Xiao, M [1 ]
机构
[1] Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA
[2] Univ Arkansas, Dept Chem & Biochem, Fayetteville, AR 72701 USA
关键词
D O I
10.1021/nl0342491
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
We report our experimental studies of surface-related emission in highly luminescent CdSe quantum dots (QDs) with controlled quantum yield and photooxidation by time-resolved photoluminescence measurements. This kind of surface-related emission, with a radiative lifetime of tens of nanoseconds, implies the involvement of surface states in the carrier recombination process of such highly luminescent CdSe QDs.
引用
收藏
页码:1103 / 1106
页数:4
相关论文
共 28 条
[11]   Quantum correlation among photons from a single quantum dot at room temperature [J].
Michler, P ;
Imamoglu, A ;
Mason, MD ;
Carson, PJ ;
Strouse, GF ;
Buratto, SK .
NATURE, 2000, 406 (6799) :968-970
[12]   FLUORESCENCE-LINE NARROWING IN CDSE QUANTUM DOTS - SURFACE LOCALIZATION OF THE PHOTOGENERATED EXCITON [J].
NIRMAL, M ;
MURRAY, CB ;
BAWENDI, MG .
PHYSICAL REVIEW B, 1994, 50 (04) :2293-2300
[13]   DYNAMICS OF ELECTRON-HOLE PAIR RECOMBINATION IN SEMICONDUCTOR CLUSTERS [J].
ONEIL, M ;
MAROHN, J ;
MCLENDON, G .
JOURNAL OF PHYSICAL CHEMISTRY, 1990, 94 (10) :4356-4363
[14]   Shape control of CdSe nanocrystals [J].
Peng, XG ;
Manna, L ;
Yang, WD ;
Wickham, J ;
Scher, E ;
Kadavanich, A ;
Alivisatos, AP .
NATURE, 2000, 404 (6773) :59-61
[15]   Epitaxial growth of highly luminescent CdSe/CdS core/shell nanocrystals with photostability and electronic accessibility [J].
Peng, XG ;
Schlamp, MC ;
Kadavanich, AV ;
Alivisatos, AP .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 1997, 119 (30) :7019-7029
[16]   Anti-Stokes photoluminescence in colloidal semiconductor quantum dots [J].
Poles, E ;
Selmarten, DC ;
Micic, OI ;
Nozik, AJ .
APPLIED PHYSICS LETTERS, 1999, 75 (07) :971-973
[17]   Control of photoluminescence properties of CdSe nanocrystals in growth [J].
Qu, LH ;
Peng, XG .
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2002, 124 (09) :2049-2055
[18]  
Rakovich YP, 2002, PHYS STATUS SOLIDI B, V229, P449, DOI 10.1002/1521-3951(200201)229:1<449::AID-PSSB449>3.0.CO
[19]  
2-4
[20]   Fluorescence decay time of single semiconductor nanocrystals [J].
Schlegel, G ;
Bohnenberger, J ;
Potapova, I ;
Mews, A .
PHYSICAL REVIEW LETTERS, 2002, 88 (13) :4-137401