Preparation and electrical properties of sol-gel derived (1-x)Pb(Sc1/2Nb1/2)O3-xPbTiO3 (x=0.6) thin films

被引:10
作者
Kuh, BJ [1 ]
Choo, WK [1 ]
机构
[1] Korea Adv Inst Sci & Technol, Dept Mat Sci & Engn, Yusong Gu, Taejon 305701, South Korea
关键词
ferroelectric properties; (1-x)Pb(Sc1/2Nb1/2)O-3-xPbTiO(3); sol-gel processes;
D O I
10.1016/S0955-2219(01)00052-8
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The films of (1-x)Pb(Sc1/2Nb1/2)O-3-xPbTiO(3) (x=0.6, PSNT(40/60)) were successfully deposited on Pt/Ti/SiO2/Si substrates via spin coating method. Using combination of homogeneous precursor solutions and two-step heat treatment, it was possible to obtain the PSNT(40/60) thin films of perfect perovskite phase with virtually no pyrochlore phase after annealing just above 550 degreesC. The root-mean-square surface roughness of a 240-nm-thick film was 3 nm as measured by atomic force microscope (AFM). The PSNT(40/60) films annealed at 650 degreesC showed a well-saturated hysteresis loop at an applied voltage of 7 V with remnant polarization (P-r) and coercieve voltage (V-c) of 14 muC/cm(2) and 1.5 V. The leakage current density was lower than 10(-6) A/cm(2) at an applied voltage of 7 V. (C) 2001 Elsevier Science Ltd.
引用
收藏
页码:1509 / 1512
页数:4
相关论文
共 7 条
[1]   High strain and low mechanical quality factor piezoelectric Pb[(Sc1/2Nb1/2)0.575Ti0.425]O3 ceramics [J].
Alberta, EF ;
Bhalla, AS .
MATERIALS LETTERS, 1998, 35 (3-4) :199-201
[2]   Orientation dependence of fatigue behavior in relaxor ferroelectric-PbTiO3 thin films [J].
Bornand, V ;
Trolier-McKinstry, S ;
Takemura, K ;
Randall, CA .
JOURNAL OF APPLIED PHYSICS, 2000, 87 (08) :3965-3972
[3]   Correlation between structure, microstructure, and ferroelectric properties of PbZr0.2Ti0.8O3 integrated film:: Influence of the sol-gel process and the substrate [J].
Floquet, N ;
Hector, J ;
Gaucher, P .
JOURNAL OF APPLIED PHYSICS, 1998, 84 (07) :3815-3826
[4]   Relaxor behavior and electromechanical properties of Pb(Mg1/3Nb2/3)O3 thin films [J].
Kighelman, Z ;
Damjanovic, D ;
Seifert, A ;
Sagalowicz, L ;
Setter, N .
APPLIED PHYSICS LETTERS, 1998, 73 (16) :2281-2283
[5]   Top-interface-controlled switching and fatigue endurance of (Pb, La)(Zr,Ti)O3 ferroelectric capacitors [J].
Stolichnov, I ;
Tagantsev, A ;
Setter, N ;
Cross, JS ;
Tsukada, M .
APPLIED PHYSICS LETTERS, 1999, 74 (23) :3552-3554
[6]   Dielectric properties of pulsed laser deposited films of PbMg1/3Nb2/3-PbTiO3 and PbSc1/2Nb1/2O3-PbTiO3 relaxor ferroelectrics [J].
Tyunina, M ;
Levoska, J ;
Sternberg, A ;
Leppävuori, S .
JOURNAL OF APPLIED PHYSICS, 1999, 86 (09) :5179-5184
[7]   IMPROVED FERROELECTRIC PROPERTIES OF NIOBIUM-DOPED PB[(SC1/2NB1/2)TI]O3 CERAMIC MATERIAL [J].
YAMASHITA, Y .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 1-REGULAR PAPERS BRIEF COMMUNICATIONS & REVIEW PAPERS, 1993, 32 (11A) :5036-5040