Hexathienoacene: Synthesis, Characterization, and Thin-Film Transistors

被引：24

作者：

Liu, Ying ^{[1
,2
]}

Sun, Xiangnan ^{[1
,2
]}

Di, Chong-an ^{[1
]}

Liu, Yunqi ^{[1
]}

Du, Chunyan ^{[1
,2
]}

Lu, Kun ^{[1
]}

Ye, Shanghui ^{[1
,2
]}

Yu, Gui ^{[1
]}

机构：

[1] Chinese Acad Sci, Inst Chem, Key Lab Organ Solids, Beijing 100190, Peoples R China

[2] Chinese Acad Sci, Grad Sch, Beijing 100039, Peoples R China

来源：

CHEMISTRY-AN ASIAN JOURNAL | 2010年 / 5卷 / 07期

基金：

中国国家自然科学基金;

关键词：

acenes; conjugation; density functional calculations; sulfur; transistors; HIGH-PERFORMANCE; ORGANIC SEMICONDUCTOR; HIGH-MOBILITY; ACENES; OLIGOTHIOPHENES; HETEROACENES; DERIVATIVES; PENTACENE; STABILITY; SINGLET;

D O I：

10.1002/asia.201000001

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A new linear six thiophene-fused system of hexathienoacene (HTA) has been synthesized, which has also been compared with pentathienoacene (PTA) in terms of optical, electrochemical, and charge-transfer properties of organic semiconductors. The highest mobility of 0.06 cm2 V-1 s-1 with a current on/off ratio of 105 on n-octadecyltrichlorosilane (OTS)-treated SiO2/Si substrates has been achieved. © 2010 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

引用

页码：1550 / 1554

页数：5

共 42 条

[31] Advances in organic field-effect transistors [J].

Sun, YM ;

Liu, YQ ;

Zhu, DB .

JOURNAL OF MATERIALS CHEMISTRY, 2005, 15 (01) :53-65

[32]

Thelakkat M, 1998, ADV MATER, V10, P219, DOI 10.1002/(SICI)1521-4095(199802)10:3<219::AID-ADMA219>3.0.CO

[33]

2-6

[34] Naphthyl end-capped quarterthiophene: A simple organic semiconductor with high mobility and air stability [J].

Tian, Hongkun ;

Shi, Jianwu ;

Yan, Donghang ;

Wang, Lixiang ;

Geng, Yanhou ;

Wang, Fosong .

ADVANCED MATERIALS, 2006, 18 (16) :2149-+

[35] Steady-state and time-resolved studies of 2,7-carbazole-based conjugated polymers in solution and as thin films:: determination of their solid state fluorescence quantum efficiencies [J].

Tirapattur, S ;

Belletête, M ;

Drolet, N ;

Leclerc, M ;

Durocher, G .

CHEMICAL PHYSICS LETTERS, 2003, 370 (5-6) :799-804

[36] Synthesis and characterization of anthra[2,3-b]thiophene and tetraceno[2,3-b]thiophenes for organic field-effect transistor applications [J].

Valiyev, Famil ;

Hu, Wei-Shan ;

Chen, Hsing-Yin ;

Kuo, Ming-Ytt ;

Chao, Ito ;

Tao, Yu-Tai .

CHEMISTRY OF MATERIALS, 2007, 19 (12) :3018-3026

[37] Progress and perspective of polymer white light-emitting devices and materials [J].

Wu, Hongbin ;

Ying, Lei ;

Yang, Wei ;

Cao, Yong .

CHEMICAL SOCIETY REVIEWS, 2009, 38 (12) :3391-3400

[38] Indolo[3,2-b]carbazole-based thin-film transistors with high mobility and stability [J].

Wu, YL ;

Li, YN ;

Gardner, S ;

Ong, BS .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2005, 127 (02) :614-618

[39] A highly π-stacked organic semiconductor for field-effect transistors based on linearly condensed pentathienoacene [J].

Xiao, K ;

Liu, YQ ;

Qi, T ;

Zhang, W ;

Wang, F ;

Gao, JH ;

Qiu, WF ;

Ma, YQ ;

Cui, GL ;

Chen, SY ;

Zhan, XW ;

Yu, G ;

Qin, JG ;

Hu, WP ;

Zhu, DB .

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY, 2005, 127 (38) :13281-13286

[40] Ring fusion effects on the solid-state properties of α-oligothiophenes [J].

Zhang, Xinnan ;

Johnson, James P. ;

Kampf, Jeff W. ;

Matzger, Adam J. .

CHEMISTRY OF MATERIALS, 2006, 18 (15) :3470-3476

← 1 2 3 4 5 →