Determination of the trap-assisted recombination strength in polymer light emitting diodes

被引:52
作者
Kuik, Martijn [1 ]
Nicolai, Herman T. [1 ]
Lenes, Martijn [1 ]
Wetzelaer, Gert-Jan A. H. [1 ]
Lu, Mingtao [1 ]
Blom, Paul W. M. [1 ,2 ]
机构
[1] Univ Groningen, Zernike Inst Adv Mat, NL-9747 AG Groningen, Netherlands
[2] Holst Ctr, NL-5656 AE Eindhoven, Netherlands
关键词
POLY(P-PHENYLENE VINYLENE); SOLAR-CELLS; DEPENDENCE; MOBILITY; TRANSPORT; ELECTRON; EMISSION; DEVICES;
D O I
10.1063/1.3559911
中图分类号
O59 [应用物理学];
学科分类号
摘要
The recombination processes in poly(p-phenylene vinylene) based polymer light-emitting diodes (PLEDs) are investigated. Photogenerated current measurements on PLED device structures reveal that next to the known Langevin recombination also trap-assisted recombination is an important recombination channel in PLEDs, which has not been considered until now. The dependence of the open-circuit voltage on light intensity enables us to determine the strength of this process. Numerical modeling of the current-voltage characteristics incorporating both Langevin and trap-assisted recombination yields a correct and consistent description of the PLED, without the traditional correction of the Langevin prefactor. At low bias voltage the trap-assisted recombination rate is found to be dominant over the free carrier recombination rate. (C) 2011 American Institute of Physics. [doi:10.1063/1.3559911]
引用
收藏
页数:3
相关论文
共 27 条
  • [1] LANGEVIN-TYPE CHARGE-CARRIER RECOMBINATION IN A DISORDERED HOPPING SYSTEM
    ALBRECHT, U
    BASSLER, H
    [J]. PHYSICA STATUS SOLIDI B-BASIC RESEARCH, 1995, 191 (02): : 455 - 459
  • [2] CARRIER DEEP-TRAPPING MOBILITY-LIFETIME PRODUCTS IN POLY(P-PHENYLENE VINYLENE)
    ANTONIADIS, H
    ABKOWITZ, MA
    HSIEH, BR
    [J]. APPLIED PHYSICS LETTERS, 1994, 65 (16) : 2030 - 2032
  • [3] Blom PWM, 1998, POLYM ADVAN TECHNOL, V9, P390, DOI 10.1002/(SICI)1099-1581(199807)9:7<390::AID-PAT795>3.0.CO
  • [4] 2-9
  • [5] Temperature dependent electron-hole recombination in polymer light-emitting diodes
    Blom, PWM
    deJong, MJM
    Breedijk, S
    [J]. APPLIED PHYSICS LETTERS, 1997, 71 (07) : 930 - 932
  • [6] Performance of a polymer light-emitting diode with enhanced charge carrier mobility
    Blom, PWM
    Martens, HCF
    Schoo, HEM
    Vissenberg, MCJM
    Huiberts, JN
    [J]. SYNTHETIC METALS, 2001, 122 (01) : 95 - 98
  • [7] Electron and hole transport in poly(p-phenylene vinylene) devices
    Blom, PWM
    deJong, MJM
    Vleggaar, JJM
    [J]. APPLIED PHYSICS LETTERS, 1996, 68 (23) : 3308 - 3310
  • [8] VISIBLE-LIGHT EMISSION FROM SEMICONDUCTING POLYMER DIODES
    BRAUN, D
    HEEGER, AJ
    [J]. APPLIED PHYSICS LETTERS, 1991, 58 (18) : 1982 - 1984
  • [9] Analytical model for the open-circuit voltage and its associated resistance in organic planar heterojunction solar cells
    Cheyns, D.
    Poortmans, J.
    Heremans, P.
    Deibel, C.
    Verlaak, S.
    Rand, B. P.
    Genoe, J.
    [J]. PHYSICAL REVIEW B, 2008, 77 (16):
  • [10] Hysteresis-free electron currents in poly(p-phenylene vinylene) derivatives
    Craciun, N. I.
    Zhang, Y.
    Palmaerts, A.
    Nicolai, H. T.
    Kuik, M.
    Kist, R. J. P.
    Wetzelaer, G. A. H.
    Wildeman, J.
    Vandenbergh, J.
    Lutsen, L.
    Vanderzande, D.
    Blom, P. W. M.
    [J]. JOURNAL OF APPLIED PHYSICS, 2010, 107 (12)