Scanning tunneling microscopy investigation at high temperatures of islands and holes on Si(111)7x7 in real time:: evidence for diffusion-limited decay

被引:7
作者
Hildebrandt, S
Kraus, A
Kulla, R
Wilhelmi, G
Hanbücken, M
Neddermeyer, H [1 ]
机构
[1] Univ Halle Wittenberg, Fachbereich Phys, D-06099 Halle, Germany
[2] VCH Verlag Berlin GmbH, Phys Status Solid Wiley, D-130086 Berlin, Germany
[3] Ruhr Univ Bochum, Inst Expt Phys, D-44780 Bochum, Germany
[4] CNRS, CRMC2, F-13288 Marseille, France
关键词
silicon; scanning tunneling microscopy; surface diffusion; surface structure; morphology; roughness; and topography;
D O I
10.1016/S0039-6028(01)01054-8
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
The annealing behavior of hole- and island-like nanostructures fabricated in situ in the scanning tunneling microscope on Si(111)7 x 7 has been investigated in the range from 720 to 830 K. In contrast to previous work, the analysis reveals diffusion-controlled decay kinetics to be described by a (t(0) - t)(2/3) law, From the temperature dependence of the diffusion coefficient, we obtain an activation energy of(1.49 +/- 0.12) eV which is discussed in terms of a diffusion barrier for the moving adatoms. The comparison of the decay between hole and island structures suggest a missing Ehrlich-Schwoebel barrier for hole filling. (C) 2001 Elsevier Science B.V. All rights reserved.
引用
收藏
页码:24 / 32
页数:9
相关论文
共 29 条
[1]   VARIATIONAL PHASE-SPACE THEORY STUDIES OF SILICON-ATOM DIFFUSION ON RECONSTRUCTED SI(111)-(7X7) SURFACES [J].
AGRAWAL, PM ;
THOMPSON, DL ;
RAFF, LM .
JOURNAL OF CHEMICAL PHYSICS, 1989, 91 (10) :6463-6471
[2]   BROWNIAN-MOTION OF STEPS ON SI(111) [J].
BARTELT, NC ;
GOLDBERG, JL ;
EINSTEIN, TL ;
WILLIAMS, ED ;
HEYRAUD, JC ;
METOIS, JJ .
PHYSICAL REVIEW B, 1993, 48 (20) :15453-15456
[3]   FIELD EVAPORATION BETWEEN A GOLD TIP AND A GOLD SURFACE IN THE SCANNING TUNNELING MICROSCOPE CONFIGURATION [J].
CHANG, CS ;
SU, WB ;
TSONG, TT .
PHYSICAL REVIEW LETTERS, 1994, 72 (04) :574-577
[4]   AN STM STUDY OF MECHANOCHEMICALLY PREPARED SI(111) SUBSTRATES - AN EXTENDED SET OF VICINAL SURFACES [J].
HANBUCKEN, M ;
ROTTGER, B ;
KLIESE, R ;
VIANEY, I ;
NEDDERMEYER, H .
EUROPHYSICS LETTERS, 1993, 23 (08) :573-578
[5]   IN-SITU DIRECT IMAGING OF SCANNING TUNNELING MICROSCOPE TIP APEX [J].
HEIKE, S ;
HASHIZUME, T ;
WADA, Y .
JAPANESE JOURNAL OF APPLIED PHYSICS PART 2-LETTERS & EXPRESS LETTERS, 1995, 34 (8B) :L1061-L1063
[6]   OBSERVATION OF SI(111) SURFACE-TOPOGRAPHY CHANGES DURING SI MOLECULAR-BEAM EPITAXIAL-GROWTH USING MICROPROBE REFLECTION HIGH-ENERGY ELECTRON-DIFFRACTION [J].
ICHIKAWA, M ;
DOI, T .
APPLIED PHYSICS LETTERS, 1987, 50 (17) :1141-1143
[7]   Quantitative measurements of thermal relaxation of isolated silicon hillocks and craters on the Si(111)-(7x7) surface by scanning tunneling microscopy [J].
Ichimiya, A ;
Tanaka, Y ;
Ishiyama, K .
PHYSICAL REVIEW LETTERS, 1996, 76 (25) :4721-4724
[8]   Thermal relaxation of silicon islands and craters on silicon surfaces [J].
Ichimiya, A ;
Tanaka, Y ;
Hayashi, K .
SURFACE SCIENCE, 1997, 386 (1-3) :182-194
[9]   Relaxation of nanostructures on the Si(111)(7x7) surface by high temperature scanning tunneling microscopy [J].
Ichimiya, A ;
Tanaka, Y ;
Hayashi, K .
SURFACE REVIEW AND LETTERS, 1998, 5 (3-4) :821-832
[10]   FORMATION OF NANOMETER-SCALE GROOVES IN SILICON WITH A SCANNING TUNNELING MICROSCOPE [J].
KOBAYASHI, A ;
GREY, F ;
WILLIAMS, RS ;
AONO, M .
SCIENCE, 1993, 259 (5102) :1724-1726