Tunneling broadening of vibrational sidebands in molecular transistors

被引:152
作者
Flensberg, K [1 ]
机构
[1] Cornell Univ, Atom & Solid State Phys Lab, Ithaca, NY 14853 USA
[2] Niels Bohr Inst fAPG, Orsted Lab, DK-2100 Copenhagen, Denmark
来源
PHYSICAL REVIEW B | 2003年 / 68卷 / 20期
关键词
D O I
10.1103/PhysRevB.68.205323
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
Transport through molecular quantum dots coupled to a single vibration mode is studied in the case with strong coupling to the leads. We use an expansion in the correlation between electrons on the molecule and electrons in the leads, and show that the tunneling broadening is strongly suppressed by the combination of the Pauli principle and the quantization of the oscillator. As a consequence the first Frank-Condon step is sharper than the higher order ones, and its width, when compared to the bare tunneling strength, is reduced by the overlap between the ground states of the displaced and nondisplaced oscillators.
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页数:7
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共 20 条
[1]   Memory effect in a molecular quantum dot with strong electron-vibron interaction [J].
Alexandrov, AS ;
Bratkovsky, AM .
PHYSICAL REVIEW B, 2003, 67 (23)
[2]   Influence of nanomechanical properties on single-electron tunneling: A vibrating single-electron transistor [J].
Boese, D ;
Schoeller, H .
EUROPHYSICS LETTERS, 2001, 54 (05) :668-674
[3]   Vibrational sidebands and dissipative tunneling in molecular transistors [J].
Braig, S ;
Flensberg, K .
PHYSICAL REVIEW B, 2003, 68 (20)
[4]  
GLAZMAN LI, 1988, ZH EKSP TEOR FIZ, V67, P163
[5]   Nonperturbative analysis of coupled quantum dots in a phonon bath [J].
Keil, M ;
Schoeller, H .
PHYSICAL REVIEW B, 2002, 66 (15) :1553141-1553148
[6]   Zero-bias anomalies and boson-assisted tunneling through quantum dots [J].
Konig, J ;
Schoeller, H ;
Schon, G .
PHYSICAL REVIEW LETTERS, 1996, 76 (10) :1715-1718
[7]   Nonequilibrium linked cluster expansion for steady-state quantum transport [J].
Kral, P .
PHYSICAL REVIEW B, 1997, 56 (12) :7293-7303
[8]  
Kuo DMT, 2002, PHYS REV B, V66, DOI 10.1103/PhysRevB.66.085311
[9]   Kondo resonance in a single-molecule transistor [J].
Liang, WJ ;
Shores, MP ;
Bockrath, M ;
Long, JR ;
Park, H .
NATURE, 2002, 417 (6890) :725-729
[10]  
Lundin U, 2002, PHYS REV B, V66, DOI 10.1103/PhysRevB.66.075303