One-dimensional transport with dynamic disorder

被引:4
作者
Barsegov, V [1 ]
Shapir, Y
Mukamel, S
机构
[1] Univ Rochester, Dept Chem, Rochester, NY 14627 USA
[2] Univ Rochester, Dept Phys & Astron, Rochester, NY 14627 USA
来源
PHYSICAL REVIEW E | 2003年 / 68卷 / 01期
关键词
D O I
10.1103/PhysRevE.68.011101
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
We study the mean quenching time distribution and its moments in a one-dimensional N-site donor-bridge-acceptor system where all sites are coupled to a two-state jump bath for arbitrary disorder and an arbitrary ratio kappa=<k>/R of the bath jump rate R and the average hopping rate <k>. When kappaNsimilar to1, the quenching time distribution has long power-law tails even when the waiting times are exponentially distributed. These disappear for kappaN<<1 where the hopping rate self-averages on the bath relaxation time scale. In the absence of disorder or for small kappa, the mean quenching time scales linearly with N. Otherwise, we observe a power law, similar toN(1+gamma), with a crossover to linear scaling (gamma=0) for large N. Distributions of particle position, its second moment, velocity and diffusion coefficient are computed in the infinite N limit. For times longer than R-1, the dynamic disorder self-averages and the average position, velocity, and diffusion coefficient scale linearly in time.
引用
收藏
页码:14 / 111011
页数:14
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