Multiphoton ionization of dissociating D2+ molecules

被引:36
作者
Trump, C [1 ]
Rottke, H [1 ]
Sandner, W [1 ]
机构
[1] Max Born Inst, D-12489 Berlin, Germany
来源
PHYSICAL REVIEW A | 1999年 / 59卷 / 04期
关键词
D O I
10.1103/PhysRevA.59.2858
中图分类号
O43 [光学];
学科分类号
070207 ; 0803 ;
摘要
We report? the observation of probe pulse multiphoton ionization (MPI) of dissociating D-2(+) molecular ions. D-2(+) is formed by a pump light pulse through MPI of D-2 at the equilibrium internuclear separation. The ions then dissociate in a Roquet one- and two-photon channel. MPI of D-2(+) is observed as a pump-probe delay rime-dependent structure in high-resolution D+ ion kinetic energy distributions. The dependence on delay rime is caused by Coulomb repulsion of the two bare deuterons after D-2(+): MPI which changes with the internuclear separation where the ions are hit by the probe light pulse. A model calculation shows that in the experiment we probably only observe those ions dissociating in the two-photon channel. [S1050-2947(99)01304-9].
引用
收藏
页码:2858 / 2863
页数:6
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