Enhancing UV photoconductivity of ZnO nanobelt by polyacrylonitrile functionalization

被引:123
作者
He, J. H. [1 ]
Lin, Yen H.
McConney, Michael E.
Tsukruk, Vladimir V.
Wang, Zhong L.
Bao, Gang
机构
[1] Georgia Inst Technol, Sch Mat Sci & Engn, Atlanta, GA 30332 USA
[2] Georgia Inst Technol, Sch Biomed Engn, Atlanta, GA 30332 USA
基金
美国国家卫生研究院;
关键词
D O I
10.1063/1.2798390
中图分类号
O59 [应用物理学];
学科分类号
摘要
UV photodetector fabricated using a single ZnO nanobelt (NB) has shown a photoresponse enhancement up to 750 times higher than that of a bare ZnO NB after coating with similar to 20 nm plasma polymerized acrylonitrile (PP-AN) nanoscale film. The mechanism for this colossal photoconductivity is suggested as a consequence of the efficient exciton dissociation under UV illumination due to enhanced electron transfer from valence band of ZnO NB to the PP-AN and then back to the conduction band of ZnO. This process has demonstrated an easy and effective method for improving the performance of the nanowire/NB-based devices, possibly leading to supersensitive UV detector for applications in imaging, photosensing, and intrachip optical interconnects.
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页数:4
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