Magnetic correlations at graphene edges: Basis for novel spintronics devices

被引:628
作者
Yazyev, Oleg V. [1 ,2 ]
Katsnelson, M. I. [3 ]
机构
[1] Ecole Polytech Fed Lausanne, Inst Theoret Phys, CH-1015 Lausanne, Switzerland
[2] Inst Romand Rech Numer Phys Mat, IRRMA, CH-1015 Lausanne, Switzerland
[3] Radboud Univ Nijmegen, Inst Mol & Mat, NL-6525 ED Nijmegen, Netherlands
关键词
D O I
10.1103/PhysRevLett.100.047209
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Magnetic zigzag edges of graphene are considered as a basis for novel spintronics devices despite the fact that no true long-range magnetic order is possible in one dimension. We study the transverse and longitudinal fluctuations of magnetic moments at zigzag edges of graphene from first principles. We find a high value for the spin wave stiffness D=2100 meV angstrom(2) and a spin-collinear domain wall creation energy E-dw=114 meV accompanied by low magnetic anisotropy. Above the crossover temperature T-x approximate to 10 K, the spin correlation length xi proportional to T-1 limits the long-range magnetic order to similar to 1 nm at 300 K while below T-x, it grows exponentially with decreasing temperature. We discuss possible ways of increasing the range of magnetic order and effects of edge roughness on it.
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页数:4
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共 37 条
[21]   Strong suppression of weak localization in graphene [J].
Morozov, S. V. ;
Novoselov, K. S. ;
Katsnelson, M. I. ;
Schedin, F. ;
Ponomarenko, L. A. ;
Jiang, D. ;
Geim, A. K. .
PHYSICAL REVIEW LETTERS, 2006, 97 (01)
[22]   Edge state in graphene ribbons: Nanometer size effect and edge shape dependence [J].
Nakada, K ;
Fujita, M ;
Dresselhaus, G ;
Dresselhaus, MS .
PHYSICAL REVIEW B, 1996, 54 (24) :17954-17961
[23]   Fully unconstrained approach to noncollinear magnetism: Application to small Fe clusters [J].
Oda, T ;
Pasquarello, A ;
Car, R .
PHYSICAL REVIEW LETTERS, 1998, 80 (16) :3622-3625
[24]   π-Electron ferromagnetism in metal-free carbon probed by soft x-ray dichroism [J].
Ohldag, H. ;
Tyliszczak, T. ;
Hoehne, R. ;
Spemann, D. ;
Esquinazi, P. ;
Ungureanu, M. ;
Butz, T. .
PHYSICAL REVIEW LETTERS, 2007, 98 (18)
[25]  
Perdew JP, 1997, PHYS REV LETT, V78, P1396, DOI 10.1103/PhysRevLett.77.3865
[26]   STUDY OF LINEWIDTHS OF ELECTRON SPIN RESONANCE SPECTRA OF SOME AROMATIC HYDROCARBON RADICAL IONS [J].
SEGAL, BG ;
REYMOND, A ;
FRAENKEL, GK .
JOURNAL OF CHEMICAL PHYSICS, 1969, 51 (04) :1336-&
[27]   The SIESTA method for ab initio order-N materials simulation [J].
Soler, JM ;
Artacho, E ;
Gale, JD ;
García, A ;
Junquera, J ;
Ordejón, P ;
Sánchez-Portal, D .
JOURNAL OF PHYSICS-CONDENSED MATTER, 2002, 14 (11) :2745-2779
[28]   Half-metallic graphene nanoribbons [J].
Son, Young-Woo ;
Cohen, Marvin L. ;
Louie, Steven G. .
NATURE, 2006, 444 (7117) :347-349
[29]   G TENSORS OF AROMATIC HYDROCARBONS [J].
STONE, AJ .
MOLECULAR PHYSICS, 1964, 7 (04) :311-&
[30]  
Tombros N, 2007, NATURE, V448, P571, DOI 10.1038/nature06037