Computational view of surface based organic mass spectrometry

被引：136

作者：

Garrison, Barbara J. ^{[2
]}

Postawa, Zbigniew ^{[1
]}

机构：

[1] Jagiellonian Univ, Smoluchowski Inst Phys, PL-30059 Krakow, Poland

[2] Penn State Univ, Dept Chem, University Pk, PA 16802 USA

来源：

MASS SPECTROMETRY REVIEWS | 2008年 / 27卷 / 04期

关键词：

computer simulation; molecular dynamics; atomic SIMS; cluster SIMS; MALDI;

D O I：

10.1002/mas.20165

中图分类号：

O433 [光谱学];

学科分类号：

0703 ; 070302 ;

摘要：

Surface based mass spectrometric approaches fill air important niche in the mass analysis portfolio of tools. The particular niche depends on both the underlying physics and chemistry of molecule ejection as well as experimental characteristics. In this article, we use molecular dynamics computer simulations to elucidate the fundamental processes giving rise to ejection of organic molecules in atomic and cluster secondary ion mass spectrometry (SIMS), massive cluster impact (MCI) mass spectrometry, and matrix-assisted laser desorption ionization (MALDI) mass spectrometry. This review is aimed at graduate students and experimental researchers.

引用

页码：289 / 315

页数：27

共 104 条

[41]

GARRISON BJ, 2001, TOF SIMS SURFACE ANA, P223

[42] Laser-induced molecular desorption and particle ejection from organic films [J].

Handschuh, M ;

Nettesheim, S ;

Zenobi, R .

APPLIED SURFACE SCIENCE, 1999, 137 (1-4) :125-135

[43]

HILLENKAMP F, 1991, ANAL CHEM, V63, pA1193

[44] Electrosprayed droplet impact/secondary ion mass spectrometry [J].

Hiraoka, K ;

Asakawa, D ;

Fujimaki, S ;

Takamizawa, A ;

Mori, K .

EUROPEAN PHYSICAL JOURNAL D, 2006, 38 (01) :225-229

[45] Fundamental aspects of electrospray droplet impact/SIMS [J].

Hiraoka, Kenzo ;

Mori, Kunihiko ;

Asakawa, Daiki .

JOURNAL OF MASS SPECTROMETRY, 2006, 41 (07) :894-902

[46] Microscopic mechanisms of matrix assisted laser desorption of analyte molecules: Insights from molecular dynamics simulation [J].

Itina, TE ;

Zhigilei, LV ;

Garrison, BJ .

JOURNAL OF PHYSICAL CHEMISTRY B, 2002, 106 (02) :303-310

[47]

JOHNSON RE, 1996, LARGE IONS THEIR VAP, P49

[48] CONSTRUCTION AND EVALUATION OF EMBEDDING FUNCTIONS [J].

KELCHNER, CL ;

HALSTEAD, DM ;

PERKINS, LS ;

WALLACE, NM ;

DEPRISTO, AE .

SURFACE SCIENCE, 1994, 310 (1-3) :425-435

[49] Desorption of molecules by cluster impact. A preliminary molecular dynamics study [J].

Kerford, M ;

Webb, RP .

NUCLEAR INSTRUMENTS & METHODS IN PHYSICS RESEARCH SECTION B-BEAM INTERACTIONS WITH MATERIALS AND ATOMS, 2001, 180 :44-52

[50] Molecular dynamics model of ultraviolet matrix-assisted laser desorption/ionization including ionization processes [J].

Knochenmuss, R ;

Zhigilei, LV .

JOURNAL OF PHYSICAL CHEMISTRY B, 2005, 109 (48) :22947-22957

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