Single-cycle nonlinear optics

被引:1419
作者
Goulielmakis, E. [1 ]
Schultze, M. [1 ]
Hofstetter, M. [2 ]
Yakovlev, V. S. [2 ]
Gagnon, J. [1 ]
Uiberacker, M. [2 ]
Aquila, A. L. [3 ]
Gullikson, E. M. [3 ]
Attwood, D. T. [3 ]
Kienberger, R. [1 ]
Krausz, F. [1 ,2 ]
Kleineberg, U. [2 ]
机构
[1] Max Planck Inst Quantum Opt, D-85748 Garching, Germany
[2] Univ Munich, Dept Phys, D-85748 Garching, Germany
[3] Univ Calif Berkeley, Lawrence Berkeley Lab, Ctr Xray Opt, Berkeley, CA 94720 USA
关键词
D O I
10.1126/science.1157846
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Nonlinear optics plays a central role in the advancement of optical science and laser- based technologies. We report on the confinement of the nonlinear interaction of light with matter to a single wave cycle and demonstrate its utility for time- resolved and strong- field science. The electric field of 3.3- femtosecond, 0.72- micron laser pulses with a controlled and measured waveform ionizes atoms near the crests of the central wave cycle, with ionization being virtually switched off outside this interval. Isolated sub- 100- attosecond pulses of extreme ultraviolet light ( photon energy similar to 80 electron volts), containing similar to 0.5 nanojoule of energy, emerge from the interaction with a conversion efficiency of similar to 10(-6). These tools enable the study of the precision control of electron motion with light fields and electron- electron interactions with a resolution approaching the atomic unit of time (similar to 24 attoseconds).
引用
收藏
页码:1614 / 1617
页数:4
相关论文
共 28 条
[11]   Atomic transient recorder [J].
Kienberger, R ;
Goulielmakis, E ;
Uiberacker, M ;
Baltuska, A ;
Yakovlev, V ;
Bammer, F ;
Scrinzi, A ;
Westerwalbesloh, T ;
Kleineberg, U ;
Heinzmann, U ;
Drescher, M ;
Krausz, F .
NATURE, 2004, 427 (6977) :817-821
[12]   Control of electron localization in molecular dissociation [J].
Kling, MF ;
Siedschlag, C ;
Verhoef, AJ ;
Khan, JI ;
Schultze, M ;
Uphues, T ;
Ni, Y ;
Uiberacker, M ;
Drescher, M ;
Krausz, F ;
Vrakking, MJJ .
SCIENCE, 2006, 312 (5771) :246-248
[13]   Multielectron wave-packet propagation: General theory and application [J].
Kuleff, AI ;
Breidbach, J ;
Cederbaum, LS .
JOURNAL OF CHEMICAL PHYSICS, 2005, 123 (04)
[14]   Quantum state-resolved probing of strong-field-ionized xenon atoms using femtosecond high-order harmonic transient absorption spectroscopy [J].
Loh, Zhi-Heng ;
Khalil, Munira ;
Correa, Raoul E. ;
Santra, Robin ;
Buth, Christian ;
Leone, Stephen R. .
PHYSICAL REVIEW LETTERS, 2007, 98 (14)
[15]   Amplitude and phase control of attosecond light pulses -: art. no. 033001 [J].
López-Martens, R ;
Varjú, K ;
Johnsson, P ;
Mauritsson, J ;
Mairesse, Y ;
Salières, P ;
Gaarde, MB ;
Schafer, KJ ;
Persson, A ;
Svanberg, S ;
Wahlström, CG ;
L'Huillier, A .
PHYSICAL REVIEW LETTERS, 2005, 94 (03)
[16]   Frequency-resolved optical gating for complete reconstruction of attosecond bursts -: art. no. 011401 [J].
Mairesse, Y ;
Quéré, F .
PHYSICAL REVIEW A, 2005, 71 (01)
[17]   Generation of extreme ultraviolet continuum radiation driven by a sub-10-fs two-color field [J].
Oishi, Yu ;
Kaku, Masanori ;
Suda, Akira ;
Kannari, Fumihiko ;
Midorikawa, Katsumi .
OPTICS EXPRESS, 2006, 14 (16) :7230-7237
[18]   Heterodyne mixing of laser fields for temporal gating of high-order harmonic generation [J].
Pfeifer, Thomas ;
Gallmann, Lukas ;
Abel, Mark J. ;
Nagel, Phillip M. ;
Neumark, Daniel M. ;
Leone, Stephen R. .
PHYSICAL REVIEW LETTERS, 2006, 97 (16)
[19]   An electronic time scale in chemistry [J].
Remacle, F ;
Levine, RD .
PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA, 2006, 103 (18) :6793-6798
[20]   Feynman's path-integral approach for intense-laser-atom interactions [J].
Salières, P ;
Carré, B ;
Le Déroff, L ;
Grasbon, F ;
Paulus, GG ;
Walther, H ;
Kopold, R ;
Becker, W ;
Milosevic, DB ;
Sanpera, A ;
Lewenstein, M .
SCIENCE, 2001, 292 (5518) :902-905