Monolayers at Air-Water Interfaces: From Origins-of-Life to Nanotechnology

被引：37

作者：

Ariga, Katsuhiko ^{[1
,2
]}

Hill, Jonathan P. ^{[1
,2
]}

机构：

[1] Natl Inst Mat Sci, World Premier Int Res Ctr Mat Nanoarchitecton, Tsukuba, Ibaraki 3050044, Japan

[2] Japan Sci & Technol Agcy, Tsukuba, Ibaraki 3050044, Japan

来源：

CHEMICAL RECORD | 2011年 / 11卷 / 04期

基金：

日本科学技术振兴机构;

关键词：

air-water interface; Langmuir monolayer; molecular recognition; nanotechnology; origin of life; LANGMUIR-BLODGETT-FILMS; GUANIDINIUM-FUNCTIONALIZED MONOLAYER; MESOPOROUS NANOCOMPARTMENT FILMS; CHAIN POLYPRENYL PHOSPHATES; FLAVIN ADENINE-DINUCLEOTIDE; DYNAMIC CAVITY ARRAY; BY-LAYER ADSORPTION; MOLECULAR RECOGNITION; AQUEOUS DIPEPTIDES; SUPRAMOLECULAR CHEMISTRY;

D O I：

10.1002/tcr.201100004

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The air-water interface presents several interesting features, namely a) a molecularly flat environment, b) a boundary region between two phases with different dielectric constants, c) permits or promotes dynamic interactions within the interface region, and d) a point of interaction between hydrophobic compounds and aqueous molecules. Accordingly, Langmuir monolayers at the air-water interface have several unique characteristics and properties, which require investigation. In this review-type personal account, typical examples of molecular recognition and molecular patterning at air-water interfaces are first introduced, followed by descriptions of specific and unusual properties of monolayers on water. In addition, two examples of our own results concerning Langmuir monolayers are explained. We have selected examples from two apparently unrelated research areas, these being the origin of life and future nanotechnology, in order to emphasize the diverse scientific contribution of research on monolayers at the air-water interface. DOI 10.1002/tcr.201100004

引用

页码：199 / 211

页数：13

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