Effect of laser parameters on laser ablation and laser-induced plasma formation: A numerical modeling investigation

被引:216
作者
Bogaerts, A [1 ]
Chen, ZY [1 ]
机构
[1] Univ Instelling Antwerp, Dept Chem, B-2610 Antwerp, Belgium
关键词
laser ablation; laser-induced plasma; LIBS; modeling; plume expansion; laser parameters; laser absorption;
D O I
10.1016/j.sab.2005.06.009
中图分类号
O433 [光谱学];
学科分类号
0703 ; 070302 ;
摘要
A comprehensive numerical model has recently been developed for nanosecond (ns) laser ablation of metallic targets, describing the processes of target heating, melting and vaporization, the resulting plume expansion in I arm helium gas, as well as plasma formation in the plume. In the present paper, we investigate the influence of laser parameters, i.e., laser irradiance, pulse duration and wavelength, on typical calculation results, such as the target temperature, melt and evaporation characteristics, the plume expansion velocity, plume (plasma) temperature and ionization degree, densities of neutrals, ions and electrons in the plume, as well as the laser absorption characteristics in the plume (plasma shielding). Comparison is made with experimental data from literature, whenever available, and in general, good agreement is reached between our model predictions and experimental results. Therefore, the model can be useful to predict trends in target and plume (plasma) characteristics, which are difficult to obtain experimentally. (c) 2005 Elsevier B.V. All rights reserved.
引用
收藏
页码:1280 / 1307
页数:28
相关论文
共 82 条
[51]   Nonlinear changes in plasma and crater properties during laser ablation of Si [J].
Liu, HC ;
Mao, XL ;
Yoo, JH ;
Russo, RE .
APPLIED PHYSICS LETTERS, 1999, 75 (09) :1216-1218
[52]   Thermodynamic evolution of phase explosion during high-power nanosecond laser ablation [J].
Lu, QM .
PHYSICAL REVIEW E, 2003, 67 (01) :5
[53]   Delayed phase explosion during high-power nanosecond laser ablation of silicon [J].
Lu, QM ;
Mao, SS ;
Mao, XL ;
Russo, RE .
APPLIED PHYSICS LETTERS, 2002, 80 (17) :3072-3074
[54]   Pulsed laser ablation of metals [J].
Lunney, JG ;
Jordan, R .
APPLIED SURFACE SCIENCE, 1998, 127 :941-946
[55]   Simulation of a picosecond laser ablation plasma [J].
Mao, SS ;
Mao, XL ;
Greif, R ;
Russo, RE .
APPLIED PHYSICS LETTERS, 2000, 76 (23) :3370-3372
[56]   Initiation of an early-stage plasma during picosecond laser ablation of solids [J].
Mao, SS ;
Mao, X ;
Greif, R ;
Russo, RE .
APPLIED PHYSICS LETTERS, 2000, 77 (16) :2464-2466
[57]   Laser-induced breakdown spectroscopy:: flat surface vs. cavity structurest [J].
Mao, SS ;
Zeng, XZ ;
Mao, XL ;
Russo, RE .
JOURNAL OF ANALYTICAL ATOMIC SPECTROMETRY, 2004, 19 (04) :495-498
[58]   Simulation of infrared picosecond laser-induced electron emission from semiconductors [J].
Mao, SS ;
Mao, XL ;
Greif, R ;
Russo, RE .
APPLIED SURFACE SCIENCE, 1998, 127 :206-211
[59]   Laser ablation processes investigated using inductively coupled plasma atomic emission spectroscopy (ICP-AES) [J].
Mao, XL ;
Ciocan, AC ;
Borisov, OV ;
Russo, RE .
APPLIED SURFACE SCIENCE, 1998, 127 :262-268
[60]   Enhancements in laser ablation inductively coupled plasma-atomic emission spectrometry based on laser properties and ambient environment [J].
Mao, XL ;
Borisov, OV ;
Russo, RE .
SPECTROCHIMICA ACTA PART B-ATOMIC SPECTROSCOPY, 1998, 53 (05) :731-739