Spin-Cast and Patterned Organophosphonate Self-Assembled Monolayer Dielectrics on Metal-Oxide-Activated Si

被引：66

作者：

Acton, Orb ^{[1
]}

Hutchins, Daniel ^{[1
]}

Arnadottir, Liney ^{[2
,3
]}

Weidner, Tobias ^{[2
,3
]}

Cernetic, Nathan ^{[1
]}

Ting, Guy G. ^{[4
]}

Kim, Tae-Wook ^{[1
]}

Castner, David G. ^{[2
,3
]}

Ma, Hong ^{[1
]}

Jen, Alex K. -Y. ^{[1
,4
]}

机构：

[1] Univ Washington, Dept Mat Sci & Engn, Seattle, WA 98195 USA

[2] Univ Washington, Natl ESCA & Surface Anal Ctr Biomed Problems, Dept Bioengn, Seattle, WA 98195 USA

[3] Univ Washington, Natl ESCA & Surface Anal Ctr Biomed Problems, Dept Chem Engn, Seattle, WA 98195 USA

[4] Univ Washington, Dept Chem, Seattle, WA 98195 USA

来源：

ADVANCED MATERIALS | 2011年 / 23卷 / 16期

关键词：

VOLTAGE ORGANIC TRANSISTORS; THIN-FILM TRANSISTORS; PHOSPHONIC ACID; COMPLEMENTARY CIRCUITS; SURFACE; ELECTRONICS; ALUMINUM; INTERFACE; SILICON;

D O I：

10.1002/adma.201004762

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

An efficient process is developed for modifying Si with self-assembled monolayers (SAMs) through in situ metal oxide surface activation and microcontact printing or spin-coating of phosphonic-acid-based molecules. The utility of this process is demonstrated by fabricating self-organized and solution-processed low-voltage organic thin-film transistors enabled by patterned and spincast phosphonate SAM/metal oxide hybrid dielectrics.

引用

页码：1899 / +

页数：5

共 33 条

[1] π-σ-Phosphonic Acid Organic Monolayer/Sol-Gel Hafnium Oxide Hybrid Dielectrics for Low-Voltage Organic Transistors [J].

Acton, Orb ;

Ting, Guy ;

Ma, Hong ;

Ka, Jae Won ;

Yip, Hin-Lap ;

Tucker, Neil M. ;

Jen, Alex K. -Y. .

ADVANCED MATERIALS, 2008, 20 (19) :3697-+

[2] n-Type Organic Semiconductors in Organic Electronics [J].

Anthony, John E. ;

Facchetti, Antonio ;

Heeney, Martin ;

Marder, Seth R. ;

Zhan, Xiaowei .

ADVANCED MATERIALS, 2010, 22 (34) :3876-3892

[3] Materials and Applications for Large Area Electronics: Solution-Based Approaches [J].

Arias, Ana Claudia ;

MacKenzie, J. Devin ;

McCulloch, Iain ;

Rivnay, Jonathan ;

Salleo, Alberto .

CHEMICAL REVIEWS, 2010, 110 (01) :3-24

[4] Sum-frequency vibrational spectroscopy of soluble surfactants at the air/water interface [J].

Bell, GR ;

Bain, CD ;

Ward, RN .

JOURNAL OF THE CHEMICAL SOCIETY-FARADAY TRANSACTIONS, 1996, 92 (04) :515-523

[5] Absolute molecular orientational distribution of the polystyrene surface [J].

Briggman, KA ;

Stephenson, JC ;

Wallace, WE ;

Richter, LJ .

JOURNAL OF PHYSICAL CHEMISTRY B, 2001, 105 (14) :2785-2791

[6] Patterning organic single-crystal transistor arrays [J].

Briseno, Alejandro L. ;

Mannsfeld, Stefan C. B. ;

Ling, Mang M. ;

Liu, Shuhong ;

Tseng, Ricky J. ;

Reese, Colin ;

Roberts, Mark E. ;

Yang, Yang ;

Wudl, Fred ;

Bao, Zhenan .

NATURE, 2006, 444 (7121) :913-917

[7] Acidity of the Aqueous Rutile TiO2(110) Surface from Density Functional Theory Based Molecular Dynamics [J].

Cheng, Jun ;

Sprik, Michiel .

JOURNAL OF CHEMICAL THEORY AND COMPUTATION, 2010, 6 (03) :880-889

[8] Molecular Self-Assembled Monolayers and Multilayers for Organic and Unconventional Inorganic Thin-Film Transistor Applications [J].

DiBenedetto, Sara A. ;

Facchetti, Antonio ;

Ratner, Mark A. ;

Marks, Tobin J. .

ADVANCED MATERIALS, 2009, 21 (14-15) :1407-1433

[9] Structure and Order of Phosphonic Acid-Based Self-Assembled Monolayers on Si(100) [J].

Dubey, Manish ;

Weidner, Tobias ;

Gamble, Lara J. ;

Castner, David G. .

LANGMUIR, 2010, 26 (18) :14747-14754

[10] Low-voltage organic transistors with an amorphous molecular gate dielectric [J].

Halik, M ;

Klauk, H ;

Zschieschang, U ;

Schmid, G ;

Dehm, C ;

Schütz, M ;

Maisch, S ;

Effenberger, F ;

Brunnbauer, M ;

Stellacci, F .

NATURE, 2004, 431 (7011) :963-966

← 1 2 3 4 →