Why hybrid porous solids capture greenhouse gases?

被引：559

作者：

Ferey, Gerard ^{[1
]}

Serre, Christian ^{[1
]}

Devic, Thomas ^{[1
]}

Maurin, Guillaume ^{[2
]}

Jobic, Herve ^{[3
,4
]}

Llewellyn, Philip L. ^{[5
,6
,7
]}

De Weireld, Guy ^{[8
]}

Vimont, Alexandre ^{[9
]}

Daturi, Marco ^{[9
]}

Chang, Jong-San ^{[10
]}

机构：

[1] Univ Versailles St Quentin, CNRS 8180, Inst Lavoisier, F-78035 Versailles, France

[2] Univ Montpellier 2, ENSCM, UMR CNRS UM2 5253, Inst Charles Gerhardt Montpellier, F-34095 Montpellier 05, France

[3] Univ Lyon, F-69626 Villeurbanne, France

[4] CNRS, IRCE Lyon, F-69626 Villeurbanne, France

[5] Univ Aix Marseille 1, Lab Chim Provence, CNRS, Ctr St Jerome,UMR 6264, F-13397 Marseille 20, France

[6] Univ Aix Marseille 2, Lab Chim Provence, CNRS, Ctr St Jerome,UMR 6264, F-13397 Marseille 20, France

[7] Univ Aix Marseille 3, Lab Chim Provence, CNRS, Ctr St Jerome,UMR 6264, F-13397 Marseille 20, France

[8] Fac Polytech Mons, B-7000 Mons, Belgium

[9] Univ Caen, ENSICAEN, Lab Catalyse & Spectrochim, F-14050 Caen 4, France

[10] KRICT, Catalysis Ctr Mol Engn, Taejon 305600, South Korea

来源：

CHEMICAL SOCIETY REVIEWS | 2011年 / 40卷 / 02期

关键词：

METAL-ORGANIC-FRAMEWORK; MOLECULAR-DYNAMICS SIMULATIONS; ELASTIC NEUTRON-SCATTERING; CARBON-DIOXIDE; CO2; ADSORPTION; GIANT PORES; STRUCTURAL TRANSITIONS; TRANSPORT DIFFUSIVITY; ROOM-TEMPERATURE; LINEAR ALKANES;

D O I：

10.1039/c0cs00040j

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Hybrid porous solids, with their tunable structures, their multifunctional properties and their numerous applications, are currently topical, particularly in the domain of adsorption and storage of greenhouse gases. Most of the data reported so far concern the performances of these solids in this domain, particularly in terms of adsorbed amounts of gas but do not explain at the atomic level why and how adsorption and storage occur. From a combination of structural, spectroscopic, thermodynamic experiments and of molecular simulations, this tutorial review proposes answers to these open questions with a special emphasis on CO2 and CH4 storage by some rigid and flexible hybrid porous materials.

引用

页码：550 / 562

页数：13

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