Hot STM of nanostructure dynamics on SrTiO3(001)

被引:18
作者
Marsh, H. L. [1 ]
Deak, D. S. [1 ]
Silly, F. [1 ]
Kirkland, A. I. [1 ]
Castell, M. R. [1 ]
机构
[1] Univ Oxford, Dept Mat, Oxford OX1 3PH, England
关键词
D O I
10.1088/0957-4484/17/14/031
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The dynamics of nanostructured surface phases on SrTiO3( 001) have been analysed using in situ scanning tunnelling microscopy (STM) above 800 degrees C. During high-temperature annealing, the formation, growth and ordering of the nanostructures has been observed. Dilines, with a width of similar to 1 nm, are formed from a TiO2-rich intermediary at 800 degrees C. STM during annealing at 825 degrees C has enabled us to follow both the growth and dissolution of dilines. Following extended annealing, trilines with a width of similar to 2 nm and ordered two-dimensional (2D) nano-arrays form from the diline domains. Our observations of diline dissolution implies random nucleation and growth, followed by rearrangement at elevated temperature to form domains.
引用
收藏
页码:3543 / 3548
页数:6
相关论文
共 15 条
[1]  
BECKETT P, 2002, P 7 AS PAC COMP SYST, V6, P141
[2]   Two (1 x 2) reconstructions of TiO2(110):: Surface rearrangement and reactivity studied using elevated temperature scanning tunneling microscopy [J].
Bennett, RA ;
Stone, P ;
Price, NJ ;
Bowker, M .
PHYSICAL REVIEW LETTERS, 1999, 82 (19) :3831-3834
[3]   Nanostructures on the SrTiO3(001) surface studied by STM [J].
Castell, MR .
SURFACE SCIENCE, 2002, 516 (1-2) :33-42
[4]   Nanowires of four epitaxial hexagonal silicides grown on Si(001) [J].
Chen, Y ;
Ohlberg, DAA ;
Williams, RS .
JOURNAL OF APPLIED PHYSICS, 2002, 91 (05) :3213-3218
[5]   Ordering of TiO2-based nanostructures on SrTiO3(001) surfaces [J].
Deak, DS ;
Silly, F ;
Newell, DT ;
Castell, MR .
JOURNAL OF PHYSICAL CHEMISTRY B, 2006, 110 (18) :9246-9251
[6]   The surface science of titanium dioxide [J].
Diebold, U .
SURFACE SCIENCE REPORTS, 2003, 48 (5-8) :53-229
[7]   Growth of nanowire superlattice structures for nanoscale photonics and electronics [J].
Gudiksen, MS ;
Lauhon, LJ ;
Wang, J ;
Smith, DC ;
Lieber, CM .
NATURE, 2002, 415 (6872) :617-620
[8]   Real-time STM study of inter-nanowire reactions:: GdSi2 nanowires on Si(100) [J].
Harrison, BC ;
Boland, JJ .
SURFACE SCIENCE, 2005, 594 (1-3) :93-98
[9]   High-temperature STM for atomic processes on semiconductor surfaces [J].
Iwatsuki, M ;
Sato, T ;
Yamamoto, Y .
APPLIED SURFACE SCIENCE, 1996, 92 :321-330
[10]   Quantum dot heterostructures: fabrication, properties, lasers (Review) [J].
Ledentsov, NN ;
Ustinov, VM ;
Shchukin, VA ;
Kop'ev, PS ;
Alferov, ZI ;
Bimberg, D .
SEMICONDUCTORS, 1998, 32 (04) :343-365