Addition energies and quasiparticle gap of CdSe nanocrystals

被引:35
作者
Franceschetti, A [1 ]
Zunger, A [1 ]
机构
[1] Natl Renewable Energy Lab, Golden, CO 80401 USA
关键词
D O I
10.1063/1.126150
中图分类号
O59 [应用物理学];
学科分类号
摘要
Using atomistic pseudopotential wave functions we calculate the quasiparticle gap, the optical gap and the electron and hole addition energies of CdSe nanocrystals. We find that the quasiparticle gap and the addition energies depend strongly on the dielectric constant of the surrounding material, while the optical gap is rather insensitive to the environment. We provide scaling lows for these quantities as a function of the quantum dot size, and compare our results with recent scanning tunneling spectroscopy experiments. (C) 2000 American Institute of Physics. [S0003-6951(00)02413-X].
引用
收藏
页码:1731 / 1733
页数:3
相关论文
共 12 条
[1]   Energy level tunneling spectroscopy and single electron charging in individual CdSe quantum dots [J].
Alperson, B ;
Rubinstein, I ;
Hodes, G ;
Porath, D ;
Millo, O .
APPLIED PHYSICS LETTERS, 1999, 75 (12) :1751-1753
[2]   Identification of atomic-like electronic states in indium arsenide nanocrystal quantum dots [J].
Banin, U ;
Cao, YW ;
Katz, D ;
Millo, O .
NATURE, 1999, 400 (6744) :542-544
[5]   Multiexciton spectroscopy of a single self-assembled quantum dot [J].
Dekel, E ;
Gershoni, D ;
Ehrenfreund, E ;
Spektor, D ;
Garcia, JM ;
Petroff, PM .
PHYSICAL REVIEW LETTERS, 1998, 80 (22) :4991-4994
[6]   Photoluminescence spectroscopy of single CdSe nanocrystallite quantum dots [J].
Empedocles, SA ;
Norris, DJ ;
Bawendi, MG .
PHYSICAL REVIEW LETTERS, 1996, 77 (18) :3873-3876
[7]   Short-range versus long-range electron-hole exchange interactions in semiconductor quantum dots [J].
Franceschetti, A ;
Wang, LW ;
Fu, H ;
Zunger, A .
PHYSICAL REVIEW B, 1998, 58 (20) :13367-13370
[8]   Intraband transitions in semiconductor nanocrystals [J].
Guyot-Sionnest, P ;
Hines, MA .
APPLIED PHYSICS LETTERS, 1998, 72 (06) :686-688
[9]   A single-electron transistor made from a cadmium selenide nanocrystal [J].
Klein, DL ;
Roth, R ;
Lim, AKL ;
Alivisatos, AP ;
McEuen, PL .
NATURE, 1997, 389 (6652) :699-701
[10]   Optical studies of individual InAs quantum dots in GaAs: Few-particle effects [J].
Landin, L ;
Miller, MS ;
Pistol, ME ;
Pryor, CE ;
Samuelson, L .
SCIENCE, 1998, 280 (5361) :262-264