Vacuum Rabi Splitting and Strong-Coupling Dynamics for Surface-Plasmon Polaritons and Rhodamine 6G Molecules

被引：268

作者：

Hakala, T. K. ^{[1
]}

Toppari, J. J. ^{[1
]}

Kuzyk, A. ^{[1
,2
]}

Pettersson, M. ^{[3
]}

Tikkanen, H. ^{[3
]}

Kunttu, H. ^{[3
]}

Torma, P. ^{[2
]}

机构：

[1] Univ Jyvaskyla, Nanosci Ctr, Dept Phys, FI-40014 Jyvaskyla, Finland

[2] Helsinki Univ Technol, Dept Appl Phys, FI-02015 Helsinki, Finland

[3] Univ Jyvaskyla, Nanosci Ctr, Dept Chem, FI-40014 Jyvaskyla, Finland

来源：

PHYSICAL REVIEW LETTERS | 2009年 / 103卷 / 05期

基金：

芬兰科学院;

关键词：

SINGLE QUANTUM-DOT; SEMICONDUCTOR MICROCAVITY; EXCITON; OPTICS; LIGHT;

D O I：

10.1103/PhysRevLett.103.053602

中图分类号：

O4 [物理学];

学科分类号：

0702 ;

摘要：

We report on strong coupling between surface-plasmon polaritons (SPP) and Rhodamine 6G (R6G) molecules, with double vacuum Rabi splitting energies up to 230 and 110 meV. In addition, we demonstrate the emission of all three energy branches of the strongly coupled SPP-exciton hybrid system, revealing features of system dynamics that are not visible in conventional reflectometry. Finally, in analogy to tunable-Q microcavities, we show that the Rabi splitting can be controlled by adjusting the interaction time between waveguided SPPs and R6G deposited on top of the waveguide. The interaction time can be controlled with sub-fs precision by adjusting the length of the R6G area with standard lithography methods.

引用

页数：4

共 31 条

[1] Cavity polaritons in microcavities containing disordered organic semiconductors [J].

Agranovich, VM ;

Litinskaia, M ;

Lidzey, DG .

PHYSICAL REVIEW B, 2003, 67 (08)

[2]

[Anonymous], J APPL SPECTROSC

[3] Strong coupling between surface plasmons and excitons in an organic semiconductor [J].

Bellessa, J ;

Bonnand, C ;

Plenet, JC ;

Mugnier, J .

PHYSICAL REVIEW LETTERS, 2004, 93 (03) :036404-1

[4] Concentration quenching and depolarization of rhodamine 6G in the presence of fluorescent dimers in polyvinyl alcohol films [J].

Bojarski, P .

CHEMICAL PHYSICS LETTERS, 1997, 278 (4-6) :225-232

[5] Controlling the interactions between polaritons and molecular vibrations in strongly coupled organic semiconductor microcavities [J].

Chovan, J. ;

Perakis, I. E. ;

Ceccarelli, S. ;

Lidzey, D. G. .

PHYSICAL REVIEW B, 2008, 78 (04)

[6] Strong coupling between surface plasmon-polaritons and organic molecules in subwavelength hole arrays [J].

Dintinger, J ;

Klein, S ;

Bustos, F ;

Barnes, WL ;

Ebbesen, TW .

PHYSICAL REVIEW B, 2005, 71 (03)

[7] Two-dimensional optics with surface plasmon polaritons [J].

Ditlbacher, H ;

Krenn, JR ;

Schider, G ;

Leitner, A ;

Aussenegg, FR .

APPLIED PHYSICS LETTERS, 2002, 81 (10) :1762-1764

[8]

*EPAPS, EPRLTAO103015933 EPA

[9] Plexcitonic Nanoparticles: Plasmon-Exciton Coupling in Nanoshell-J-Aggregate Complexes [J].

Fofang, Nche T. ;

Park, Tae-Ho ;

Neumann, Oara ;

Mirin, Nikolay A. ;

Nordlander, Peter ;

Halas, Naomi J. .

NANO LETTERS, 2008, 8 (10) :3481-3487

[10] Frequency conversion of propagating surface plasmon polaritons by organic molecules [J].

Hakala, T. K. ;

Toppari, J. J. ;

Pettersson, M. ;

Kuzyk, A. ;

Tikkanen, H. ;

Kunttu, H. ;

Torma, P. .

APPLIED PHYSICS LETTERS, 2008, 93 (12)

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