Resonantly driven coherent oscillations in a solid-state quantum emitter

被引:278
作者
Flagg, E. B. [1 ]
Muller, A. [2 ,3 ]
Robertson, J. W. [1 ]
Founta, S. [1 ]
Deppe, D. G. [4 ]
Xiao, M. [5 ]
Ma, W. [5 ]
Salamo, G. J. [5 ]
Shih, C. K. [1 ]
机构
[1] Univ Texas Austin, Dept Phys, Austin, TX 78712 USA
[2] NIST, Joint Quantum Inst, Gaithersburg, MD 20899 USA
[3] Univ Maryland, Gaithersburg, MD 20899 USA
[4] Univ Cent Florida, Coll Opt & Photon CREOL, Orlando, FL 32816 USA
[5] Univ Arkansas, Dept Phys, Fayetteville, AR 72701 USA
基金
美国国家科学基金会;
关键词
SPONTANEOUS EMISSION; DOT; FLUORESCENCE; PHOTONS; MICROCAVITY; MOLECULE; DEVICE;
D O I
10.1038/NPHYS1184
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
Single-quantum emitters emit only one photon at a time(1,2), but the properties of the photon depend on how the emitter is excited(3). Incoherent excitation is simple and broadly used with solid-state emitters such as quantum dots, but does not allow direct manipulation of the quantum state. Coherent, resonant excitation on the other hand is used in pump-probe techniques to examine the quantum state of the emitter(4), but does not permit collection of the single-photon emission. Coherent control with simultaneous generation of photons has been an elusive goal in solid-state approaches, where, because of strong laser scattering at the detection wavelength, measurement of resonant emission has been limited to cross-polarized detection(5) or Stokes-shift techniques(6,7). Here we demonstrate that a semiconductor quantum dot in a microcavity can be resonantly driven and its single-photon emission extracted background free. Under strong continuous-wave excitation, the dot undergoes several Rabi oscillations before emitting, which are visible as oscillations in the second-order correlation function. The quantum-dot states are therefore 'dressed', resulting in a Mollow-triplet emission spectrum. Such coherent control will be necessary for future high-efficiency sources of indistinguishable single photons(3,8), which can be used for quantum key distribution(9) or through post-selection(10) to generate entangled photon pairs(11,12).
引用
收藏
页码:203 / 207
页数:5
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