Evaluation of planar free-breathing polymer electrolyte membrane fuel cell design

被引:67
作者
Hottinen, T [1 ]
Mikkola, M [1 ]
Lund, P [1 ]
机构
[1] Helsinki Univ Technol, Lab Adv Energy Syst, FIN-02015 Helsinki, Finland
关键词
PEMFC planar design; free-breathing; current transient; small-scale application;
D O I
10.1016/j.jpowsour.2003.11.012
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A planar cell design for free-breathing fuel cell is studied. The cathode side of the cell was directly open to ambient air in a way that oxygen needed by the fuel cell reaction was provided by diffusion through the cathode side gas diffusion backing, i.e. the cell had no cathode side flow channels. The aim of the study was to demonstrate the feasibility of the cell concept by experimentally evaluating its performance with polarisation and current transient measurements. The orientation of the cell did not significantly affect the performance of the cell and signs of flooding were not observed. The maximum power density achieved in the polarisation measurements was similar to124 mW cm(-2). The current transient measurements revealed that with a small base load the cell is capable of producing momentarily current densities up to 500 mA cm(-2). The maximum transient power density achieved was similar to194 mW cm(-2) at transient current density of 450 mA cm(-2). According to the results it seems that this kind of cell design is feasible for small-scale applications, such as portable computers. (C) 2003 Elsevier B.V. All rights reserved.
引用
收藏
页码:68 / 72
页数:5
相关论文
共 9 条
[1]   Performance of polymer electrolyte membrane fuel cell (PEMFC) stacks Part I. Evaluation and simulation of an air-breathing PEMFC stack [J].
Chu, D ;
Jiang, RZ .
JOURNAL OF POWER SOURCES, 1999, 83 (1-2) :128-133
[2]   Fuel cells for low power applications [J].
Heinzel, A ;
Hebling, C ;
Müller, M ;
Zedda, M ;
Müller, C .
JOURNAL OF POWER SOURCES, 2002, 105 (02) :250-255
[3]   Effect of ambient conditions on performance and current distribution of a polymer electrolyte membrane fuel cell [J].
Hottinen, T ;
Noponen, M ;
Mennola, T ;
Himanen, O ;
Mikkola, M ;
Lund, P .
JOURNAL OF APPLIED ELECTROCHEMISTRY, 2003, 33 (3-4) :265-271
[4]   The performance of PEM fuel cells fed with oxygen through the free-convection mode [J].
Li, PW ;
Zhang, T ;
Wang, QM ;
Schaefer, L ;
Chyu, MK .
JOURNAL OF POWER SOURCES, 2003, 114 (01) :63-69
[5]   Measurement of ohmic voltage losses in individual cells of a PEMFC stack [J].
Mennola, T ;
Mikkola, M ;
Noponen, M ;
Hottinen, T ;
Lund, P .
JOURNAL OF POWER SOURCES, 2002, 112 (01) :261-272
[6]   Experimental evaluation of the dynamic behavior of an air-breathing fuel cell stack [J].
Morner, SO ;
Klein, SA .
JOURNAL OF SOLAR ENERGY ENGINEERING-TRANSACTIONS OF THE ASME, 2001, 123 (03) :225-231
[7]   Determination of mass diffusion overpotential distribution with flow pulse method from current distribution measurements in a PEMFC [J].
Noponen, M ;
Hottinen, T ;
Mennola, T ;
Mikkola, M ;
Lund, P .
JOURNAL OF APPLIED ELECTROCHEMISTRY, 2002, 32 (10) :1081-1089
[8]   Measurement of current distribution in a free-breathing PEMFC [J].
Noponen, M ;
Mennola, T ;
Mikkola, M ;
Hottinen, T ;
Lund, P .
JOURNAL OF POWER SOURCES, 2002, 106 (1-2) :304-312
[9]   Planar self-breathing fuel cells [J].
Schmitz, A ;
Tranitz, M ;
Wagner, S ;
Hahn, R ;
Hebling, C .
JOURNAL OF POWER SOURCES, 2003, 118 (1-2) :162-171