Tantalum oxide coatings as candidate environmental barriers

被引:46
作者
Moldovan, M [1 ]
Weyant, CM [1 ]
Johnson, DL [1 ]
Faber, KT [1 ]
机构
[1] Northwestern Univ, Robert R McCormick Sch Engn & Appl Sci, Dept Mat Sci & Engn, Evanston, IL 60208 USA
关键词
environmental barrier coating; plasma spray; tantalum oxide;
D O I
10.1361/10599630418103
中图分类号
TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
Tantalum (Ta) oxide, due to its high-temperature capabilities and thermal expansion coefficient similar to silicon nitride, is a promising candidate for environmental barriers for silicon (Si) nitride-based ceramics. This paper focuses on the development of plasma-sprayed Ta oxide as an environmental barrier coating for silicon nitride. Using a D-optimal design of experiments, plasma-spray processing variables were optimized to maximize coating density. The effect of processing variables on coating thickness was also determined. X-ray diffraction (XRD) was use to ascertain that the as-sprayed coatings were comprised of alpha- and beta-Ta2O5, but were fully converted to beta-Ta2O5 after a 1200 degreesC heat treatment. Grain growth of the Ta2O5 followed a time dependence of t(0.2) at 1200 degreesC.
引用
收藏
页码:51 / 56
页数:6
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