Remarkable enhancement in the dispersion and low-temperature activity of catalysts prepared via novel plasma reduction-calcination method

被引:19
作者
Liu, CJ [1 ]
Cheng, DG
Zhang, YP
Yu, KL
Xia, Q
Wang, JG
Zhu, XL
机构
[1] Tianjin Univ, Key Lab Green Chem Technol, Tianjin 300072, Peoples R China
[2] Tianjin Univ, Sch Chem Engn, Tianjin 300072, Peoples R China
[3] Tianjin Univ, ABB Plasma Greenhouse Gas Chem Lab, Tianjin 300072, Peoples R China
[4] Tianjin Univ, Dept Chem, Tianjin 300072, Peoples R China
基金
中国国家自然科学基金;
关键词
plasma; reduction; glow discharge; calcination; dispersion; acidity; stability; methane conversion;
D O I
10.1023/B:CATS.0000026991.40338.c9
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A novel plasma reduction and calcination (PR&C) method has been recently developed. Upon the experimental investigations on methane conversions, including partial oxidation, methane combustion, NO reduction by methane and CO2 reforming, the catalysts prepared by this PR&C method exhibit a remarkable enhancement in the dispersion, low-temperature activity and stability. A plasma-enhanced acidity has also been addressed, which would play an important role in the improved dispersion. The PR&C method is leading to a better preparation of supported catalysts, esp., those for methane conversion.
引用
收藏
页码:111 / 118
页数:8
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